Climate Change Data Portal
DOI | 10.1007/s11356-017-9018-1 |
Evaluation of passive sampling of gaseous mercury using different sorbing materials | |
Lin, Huiming; Zhang, Wei; Deng, Chunyan; Tong, Yingdong; Zhang, Qianggong; Wang, Xuejun | |
通讯作者 | Wang, XJ (通讯作者) |
发表日期 | 2017 |
ISSN | 0944-1344 |
EISSN | 1614-7499 |
起始页码 | 14190 |
结束页码 | 14197 |
卷号 | 24期号:16 |
英文摘要 | Atmospheric mercury monitoring is essential because of its potential human health and ecological impacts. Current automated monitoring systems include limitations such as high cost, complicated configuration, and electricity requirements. Passive samplers require no electric power and are more appropriate for screening applications and long-term monitoring. Sampling rate is a major factor to evaluate the performance of a passive sampler. In this study, laboratory experiments were carried out using an exposure chamber to search for high efficiency sorbents for gaseous mercury. Four types of sorbents, including sulfur-impregnated carbon (SIC), chlorine-impregnated carbon (CIC), bromine-impregnated carbon (BIC), and gold-coated sand (GCS) were evaluated under a wide range of meteorological parameters, including temperature, relative humidity, and wind speed. The results showed that the four sorbents all have a high sampling rate above 0.01 m(3)g(-1) day(-1), and wind speed has a positive correlation with the sampling rate. Under different temperature and relative humidity, the sampling rate of SIC keeps stable. The sampling rate of CIC and BIC shows a negative correlation with temperature, and GCS is influenced by all the three meteorological factors. Furthermore, long-term experiments were carried out to investigate the uptake capacity of GCS and SIC. Uptake curves show that the mass amount of sorbent in a passive sampler can influence uptake capacity. In the passive sampler, 0.9 g SIC or 0.9 g GCS can achieve stable uptake efficiency for at least 110 days with gaseous mercury concentration at or below 2 ng/m(3). For mercury concentration at or below 21 ng/m(3), 0.9 g SIC can maintain stable uptake efficiency for 70 days, and 0.9 g GCS can maintain stability for 45 days. |
关键词 | PERSISTENT ORGANIC POLLUTANTSIMPREGNATED ACTIVATED CARBONATMOSPHERIC MERCURYELEMENTAL MERCURYMETEOROLOGICAL FACTORSDRY DEPOSITIONAIR SAMPLERSAMBIENT AIRADSORPTIONCHINA |
英文关键词 | Passive sampler; Gaseous mercury; Sampling rate; Sorbing material; Uptake curve |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology |
WOS类目 | Environmental Sciences |
WOS记录号 | WOS:000402748300026 |
来源期刊 | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
![]() |
来源机构 | 中国科学院青藏高原研究所 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/259014 |
推荐引用方式 GB/T 7714 | Lin, Huiming,Zhang, Wei,Deng, Chunyan,et al. Evaluation of passive sampling of gaseous mercury using different sorbing materials[J]. 中国科学院青藏高原研究所,2017,24(16). |
APA | Lin, Huiming,Zhang, Wei,Deng, Chunyan,Tong, Yingdong,Zhang, Qianggong,&Wang, Xuejun.(2017).Evaluation of passive sampling of gaseous mercury using different sorbing materials.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,24(16). |
MLA | Lin, Huiming,et al."Evaluation of passive sampling of gaseous mercury using different sorbing materials".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 24.16(2017). |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。