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DOI | 10.1021/es9030408 |
Historical Reconstruction of Mercury Pollution Across the Tibetan Plateau Using Lake Sediments | |
Yang, Handong; Battarbee, Richard W.; Turner, Simon D.; Rose, Neil L.; Derwent, Richard G.; Wu, Guangjian; Yang, Ruiqiang | |
通讯作者 | Yang, HD (通讯作者) |
发表日期 | 2010 |
ISSN | 0013-936X |
EISSN | 1520-5851 |
起始页码 | 2918 |
结束页码 | 2924 |
卷号 | 44期号:8 |
英文摘要 | The Tibetan Plateau is described as the Roof of the World averaging over 4000 m above sea level; it is remote, isolated, and presumed to be a pristine region. In order to study the history of atmospheric mercury (Hg) pollution and its spatial variation across the Plateau, lakes were chosen from three areas forming a north to south transect Sediment cores were taken from three sites in each area and dated using the radionuclides Pb-210 and Cs-137. Analysis of the cores yielded the first comprehensive Hg reconstructions for the Plateau, showing clear Hg pollution at all sites. The first indication of Hg pollution is much earlier than the onset of the industrial revolution in Europe, but the most significant pollution increase is from the 1970s, followed by a further marked increase from the 1990s. The mean post-2000 atmospheric pollution Hg accumulation rates for the sampling sites were estimated at between 5.1 and 7.9 mu g m(-2) yr(-1). The increase in Hg pollution over the last few decades is synchronous with the recent economic development in Asia (especially China and India), and pollution Hg levels continue to increase. Furthermore, contemporary sediment Hg accumulation rate data are in broad agreement with Hg deposition values derived from global models that attribute pollution to sources mainly within southeast Asia. As most of the sites are exceptionally remote and situated above the atmospheric boundary layer, these results underline the need to understand the local Hg cycle in both regional and global context. |
关键词 | GASEOUS MERCURYATMOSPHERIC DEPOSITIONTROPOSPHERIC OZONEEMISSIONACCUMULATIONTRANSPORTAIRCHEMISTRYRATESSNOW |
语种 | 英语 |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS记录号 | WOS:000276556000029 |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
来源机构 | 中国科学院青藏高原研究所 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/257779 |
推荐引用方式 GB/T 7714 | Yang, Handong,Battarbee, Richard W.,Turner, Simon D.,et al. Historical Reconstruction of Mercury Pollution Across the Tibetan Plateau Using Lake Sediments[J]. 中国科学院青藏高原研究所,2010,44(8). |
APA | Yang, Handong.,Battarbee, Richard W..,Turner, Simon D..,Rose, Neil L..,Derwent, Richard G..,...&Yang, Ruiqiang.(2010).Historical Reconstruction of Mercury Pollution Across the Tibetan Plateau Using Lake Sediments.ENVIRONMENTAL SCIENCE & TECHNOLOGY,44(8). |
MLA | Yang, Handong,et al."Historical Reconstruction of Mercury Pollution Across the Tibetan Plateau Using Lake Sediments".ENVIRONMENTAL SCIENCE & TECHNOLOGY 44.8(2010). |
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