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DOI10.1016/j.atmosenv.2009.06.023
Concentrations, seasonal variations, and transport of carbonaceous aerosols at a remote Mountainous region in western China
Cao, Jun-Ji; Xu, Bai-Qing; He, Jian-Qiao; Liu, Xian-Qin; Han, Yong-Ming; Wang, Ge-hui; Zhu, Chong-shu
通讯作者Cao, JJ (通讯作者)
发表日期2009
ISSN1352-2310
EISSN1873-2844
起始页码4444
结束页码4452
卷号43期号:29
英文摘要Carbonaceous aerosol concentrations were determined for total suspended particle samples collected from Muztagh Ata Mountain in western China from December 2003 to February 2006. Elemental carbon (EC) varied from 0.004 to 0.174 mu g m(-3) (average = 0.055 mu g m(-3)) while organic carbon (OC) ranged from 0.12 to 2.17 mu g m(-3) and carbonate carbon (CC) from below detection to 3.57 mu g m(-3). Overall, EC was the least abundant fraction of carbonaceous species, and the EC concentrations approached those in some remote polar areas, possibly representing a regional background. Low EC and OC concentrations occurred in winter and spring while high CC in spring and summer was presumably due to dust from the Taklimakan desert, China. OC/EC ratios averaged 10.0, and strong correlations between OC and EC in spring-winter suggest their cycles are coupled, but lower correlations in summer-autumn suggest influences from biogenic OC emissions and secondary OC formation. Trajectory analyses indicate that air transported from outside of China brings similar to 0.05 mu g m(-3) EC, similar to 0.42 mu g m(-3) OC, and similar to 0.10 mu g m(-3) CC to the site, with higher levels coming from inside China. The observed EC was within the range of loadings estimated from a glacial ice core, and implications of EC-induced warming for regional climate and glacial ice dynamics are discussed. (C) 2009 Elsevier Ltd. All rights reserved.
关键词ELEMENTAL CARBONBLACK CARBONNORTHERN CHINADUSTTEMPERATUREMUZTAGATACLIMATEPM(2.5)STATIONRECORD
英文关键词Elemental carbon; Organic carbon; Carbonate carbon; Aerosol; Ice core; Remote atmosphere
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000269421200008
来源期刊ATMOSPHERIC ENVIRONMENT
来源机构中国科学院青藏高原研究所
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/257648
推荐引用方式
GB/T 7714
Cao, Jun-Ji,Xu, Bai-Qing,He, Jian-Qiao,et al. Concentrations, seasonal variations, and transport of carbonaceous aerosols at a remote Mountainous region in western China[J]. 中国科学院青藏高原研究所,2009,43(29).
APA Cao, Jun-Ji.,Xu, Bai-Qing.,He, Jian-Qiao.,Liu, Xian-Qin.,Han, Yong-Ming.,...&Zhu, Chong-shu.(2009).Concentrations, seasonal variations, and transport of carbonaceous aerosols at a remote Mountainous region in western China.ATMOSPHERIC ENVIRONMENT,43(29).
MLA Cao, Jun-Ji,et al."Concentrations, seasonal variations, and transport of carbonaceous aerosols at a remote Mountainous region in western China".ATMOSPHERIC ENVIRONMENT 43.29(2009).
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