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DOI | 10.1016/j.envpol.2020.116000 |
Light absorption and fluorescence characteristics of water-soluble organic compounds in carbonaceous particles at a typical remote site in the southeastern Himalayas and Tibetan Plateau | |
Zhang, Chao; Chen, Meilian; Kang, Shichang; Yan, Fangping; Han, Xiaowen; Gautam, Sangita; Hu, Zhaofu; Zheng, Huijun; Chen, Pengfei; Gao, Shaopeng; Wang, Pengling; Li, Chaoliu | |
通讯作者 | Li, CL (通讯作者),Chinese Acad Sci, Inst Tibetan Plateau Res, CAS Key Lab Tibetan Environm Changes & Land Surfa, Beijing 100101, Peoples R China. |
发表日期 | 2021 |
ISSN | 0269-7491 |
EISSN | 1873-6424 |
卷号 | 272 |
英文摘要 | Carbonaceous particles play an important role in climate change, and an increase in their emission and deposition causes glacier melting in the Himalayas and the Tibetan Plateau (HTP). This implies that studying their basic characteristics is crucial for a better understanding of the climate forcing observed in this area. Thus, we investigated characteristics of carbonaceous particles at a typical remote site of southeastern HTP. Organic carbon and elemental carbon concentrations at this study site were 1.86 +/- 0.84 and 0.18 +/- 0.09 mu g m(-3), respectively, which are much lower than those reported for other frequently monitored stations in the same region. Thus, these values reflect the background characteristics of the study site. Additionally, the absorption coefficient per mass (alpha/rho) of water-soluble organic carbon (WSOC) at 365 nm was 0.60 +/- 0.19 m(2) g(-1), with the highest and lowest values corresponding to the winter and monsoon seasons, respectively. Multi-dimensional fluorescence analysis showed that the WSOC consisted of approximately 37% and 63% protein and humic-like components, respectively, and the latter was identified as the component that primarily determined the light absorption ability of the WSOC, which also showed a significant relationship with some major ions, including SO42-, K+, and Ca2+, indicating that combustion activities as well as mineral dust were two important contributors to WSOC at the study site. (C) 2020 Elsevier Ltd. All rights reserved. |
英文关键词 | Water-soluble organic carbon; Light absorption; Fluorescence components; Himalayas and Tibetan plateau |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology |
WOS类目 | Environmental Sciences |
WOS记录号 | WOS:000615555000061 |
来源期刊 | ENVIRONMENTAL POLLUTION |
来源机构 | 中国科学院西北生态环境资源研究院 |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/255086 |
作者单位 | [Zhang, Chao; Han, Xiaowen; Gautam, Sangita; Gao, Shaopeng; Li, Chaoliu] Chinese Acad Sci, Inst Tibetan Plateau Res, CAS Key Lab Tibetan Environm Changes & Land Surfa, Beijing 100101, Peoples R China; [Chen, Meilian] Guangdong Technion Israel Inst Technol, Environm Program, Shantou 515063, Peoples R China; [Kang, Shichang; Yan, Fangping; Hu, Zhaofu; Zheng, Huijun; Chen, Pengfei; Li, Chaoliu] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China; [Kang, Shichang; Li, Chaoliu] Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China; [Zhang, Chao; Kang, Shichang; Gautam, Sangita; Hu, Zhaofu; Zheng, Huijun] Univ Chinese Acad Sci, Beijing 100049, Peoples R China; [Yan, Fangping] Lappeenranta Univ Technol, LUT Sch Engn Sci, POB 20, Lappeenranta 53851, Finland; [Han, Xiaowen] Guilin Univ Technol, Coll Geomat & Geoinformat, 12 Jiangan Rd, Guilin 541004, Peoples R China; [Wang, Pengling] Natl Climate Ctr, China... |
推荐引用方式 GB/T 7714 | Zhang, Chao,Chen, Meilian,Kang, Shichang,et al. Light absorption and fluorescence characteristics of water-soluble organic compounds in carbonaceous particles at a typical remote site in the southeastern Himalayas and Tibetan Plateau[J]. 中国科学院西北生态环境资源研究院,2021,272. |
APA | Zhang, Chao.,Chen, Meilian.,Kang, Shichang.,Yan, Fangping.,Han, Xiaowen.,...&Li, Chaoliu.(2021).Light absorption and fluorescence characteristics of water-soluble organic compounds in carbonaceous particles at a typical remote site in the southeastern Himalayas and Tibetan Plateau.ENVIRONMENTAL POLLUTION,272. |
MLA | Zhang, Chao,et al."Light absorption and fluorescence characteristics of water-soluble organic compounds in carbonaceous particles at a typical remote site in the southeastern Himalayas and Tibetan Plateau".ENVIRONMENTAL POLLUTION 272(2021). |
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