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DOI10.3390/atmos12040456
Water-Soluble Ions in Atmospheric Aerosol Measured in a Semi-Arid and Chemical-Industrialized City, Northwest China
Jiang, Huimin; Li, Zhongqin; Wang, Feiteng; Zhou, Xi; Wang, Fanglong; Ma, Shan; Zhang, Xin
通讯作者Li, ZQ (通讯作者),Northwest Normal Univ, Coll Geog & Environm Sci, Lanzhou 730000, Peoples R China. ; Li, ZQ (通讯作者),Chinese Acad Sci, Tianshan Glaciol Stn, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China. ; Li, ZQ (通讯作者),Shihezi Univ, Coll Sci, Shihezi 832000, Peoples R China.
发表日期2021
EISSN2073-4433
卷号12期号:4
英文摘要We investigated water-soluble ions (WSIs) of aerosol samples collected from 2016 to 2017 in Lanzhou, a typical semi-arid and chemical-industrialized city in Northwest China. WSIs concentration was higher in the heating period (35.68 +/- 19.17 mu g/m(3)) and lower in the non-heating period (12.45 +/- 4.21 mu g/m(3)). NO3-, SO42-, NH4+ and Ca2+ were dominant WSIs. The concentration of SO42- has decreased in recent years, while the NO3- level was increasing. WSIs concentration was affected by meteorological factors. The sulfur oxidation and nitrogen oxidation ratios (SOR and NOR) exceeded 0.1, inferring the vital contribution of secondary transformation. Meanwhile higher O-3 concentration and temperature promoted the homogeneous reaction of SO2. Lower temperature and high relative humidity (RH) were more suitable for heterogeneous reactions of NO2. Three-phase cluster analysis illustrated that the anthropogenic source ions and natural source ions were dominant WSIs during the heating and non-heating periods, respectively. The backward trajectory analysis and the potential source contribution function model indicated that Lanzhou was strongly influenced by the Hexi Corridor, northeastern Qinghai-Tibetan Plateau, northern Qinghai province, Inner Mongolia Plateau and its surrounding cities. This research will improve our understanding of the air quality and pollutant sources in the industrial environment.
关键词SOURCE APPORTIONMENTAIR-POLLUTIONPARTICULATE MATTERNITRATE FORMATIONINORGANIC-IONSDUST SOURCESPM2.5HAZECOMPONENTSPARTICLES
英文关键词total suspended particulates (TSP); water-soluble ions (WSIs); formation mechanism; source identification; Lanzhou
语种英语
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000642726200001
来源期刊ATMOSPHERE
来源机构中国科学院西北生态环境资源研究院
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/254380
作者单位[Jiang, Huimin; Li, Zhongqin] Northwest Normal Univ, Coll Geog & Environm Sci, Lanzhou 730000, Peoples R China; [Li, Zhongqin; Wang, Feiteng; Wang, Fanglong; Zhang, Xin] Chinese Acad Sci, Tianshan Glaciol Stn, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China; [Li, Zhongqin] Shihezi Univ, Coll Sci, Shihezi 832000, Peoples R China; [Zhou, Xi; Ma, Shan] Lanzhou Univ, Coll Earth & Environm Sci, Minist Educ, Key Lab Western Chinas Environm Syst, Lanzhou 730000, Peoples R China
推荐引用方式
GB/T 7714
Jiang, Huimin,Li, Zhongqin,Wang, Feiteng,et al. Water-Soluble Ions in Atmospheric Aerosol Measured in a Semi-Arid and Chemical-Industrialized City, Northwest China[J]. 中国科学院西北生态环境资源研究院,2021,12(4).
APA Jiang, Huimin.,Li, Zhongqin.,Wang, Feiteng.,Zhou, Xi.,Wang, Fanglong.,...&Zhang, Xin.(2021).Water-Soluble Ions in Atmospheric Aerosol Measured in a Semi-Arid and Chemical-Industrialized City, Northwest China.ATMOSPHERE,12(4).
MLA Jiang, Huimin,et al."Water-Soluble Ions in Atmospheric Aerosol Measured in a Semi-Arid and Chemical-Industrialized City, Northwest China".ATMOSPHERE 12.4(2021).
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