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DOI10.1038/s41467-021-21108-4
Ultra-fast charging in aluminum-ion batteries: electric double layers on active anode
Shen X.; Sun T.; Yang L.; Krasnoslobodtsev A.; Sabirianov R.; Sealy M.; Mei W.-N.; Wu Z.; Tan L.
发表日期2021
ISSN2041-1723
卷号12期号:1
英文摘要With the rapid iteration of portable electronics and electric vehicles, developing high-capacity batteries with ultra-fast charging capability has become a holy grail. Here we report rechargeable aluminum-ion batteries capable of reaching a high specific capacity of 200 mAh g−1. When liquid metal is further used to lower the energy barrier from the anode, fastest charging rate of 104 C (duration of 0.35 s to reach a full capacity) and 500% more specific capacity under high-rate conditions are achieved. Phase boundaries from the active anode are believed to encourage a high-flux charge transfer through the electric double layers. As a result, cationic layers inside the electric double layers responded with a swift change in molecular conformation, but anionic layers adopted a polymer-like configuration to facilitate the change in composition. © 2021, The Author(s).
语种英语
scopus关键词aluminum; lithium ion; metal; polymer; aluminum; electric vehicle; electrical method; electrode; flux measurement; fuel cell; liquid; Article; chemical composition; conformation; electric potential; electricity; liquid; surface property
来源期刊Nature Communications
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/251519
作者单位School of Aerospace, Dalian University of Technology, Dalian, 116024, China; Department of Mechanical & Materials Engineering, University of Nebraska, Lincoln, NE 68588, United States; Department of Physics, University of Nebraska, Omaha, NE 68182, United States; Nebraska Center for Materials and Nanoscience, University of Nebraska, Lincoln, NE 68588, United States
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Shen X.,Sun T.,Yang L.,et al. Ultra-fast charging in aluminum-ion batteries: electric double layers on active anode[J],2021,12(1).
APA Shen X..,Sun T..,Yang L..,Krasnoslobodtsev A..,Sabirianov R..,...&Tan L..(2021).Ultra-fast charging in aluminum-ion batteries: electric double layers on active anode.Nature Communications,12(1).
MLA Shen X.,et al."Ultra-fast charging in aluminum-ion batteries: electric double layers on active anode".Nature Communications 12.1(2021).
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