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DOI10.1038/s41467-021-27484-1
Secondary organic aerosol association with cardiorespiratory disease mortality in the United States
Pye H.O.T.; Ward-Caviness C.K.; Murphy B.N.; Appel K.W.; Seltzer K.M.
发表日期2021
ISSN2041-1723
卷号12期号:1
英文摘要Fine particle pollution, PM2.5, is associated with increased risk of death from cardiorespiratory diseases. A multidecadal shift in the United States (U.S.) PM2.5 composition towards organic aerosol as well as advances in predictive algorithms for secondary organic aerosol (SOA) allows for novel examinations of the role of PM2.5 components on mortality. Here we show SOA is strongly associated with county-level cardiorespiratory death rates in the U.S. independent of the total PM2.5 mass association with the largest associations located in the southeastern U.S. Compared to PM2.5, county-level variability in SOA across the U.S. is associated with 3.5× greater per capita county-level cardiorespiratory mortality. On a per mass basis, SOA is associated with a 6.5× higher rate of mortality than PM2.5, and biogenic and anthropogenic carbon sources both play a role in the overall SOA association with mortality. Our results suggest reducing the health impacts of PM2.5 requires consideration of SOA. © 2021, This is a U.S. Government work and not under copyright protection in the US; foreign copyright protection may apply.
语种英语
scopus关键词aerosol; anthropogenic source; carbon emission; mortality; particulate matter; United States; carbon; adverse event; aerosol; air pollutant; air pollution; environmental exposure; epidemiology; heart disease; human; mortality; pollution; respiratory tract disease; United States; Aerosols; Air Pollutants; Air Pollution; Carbon; Environmental Exposure; Environmental Pollution; Heart Diseases; Humans; Respiratory Tract Diseases; United States
来源期刊Nature Communications
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/251281
作者单位Office of Research and Development, U.S. Environmental Protection Agency, 109 TW Alexander Dr, Research Triangle Park, NC 27711, United States; Office of Research and Development, U.S. Environmental Protection Agency, 104 Mason Farm Rd, Chapel Hill, NC 27514, United States; Oak Ridge Institute for Science and Education Postdoctoral Fellow in the Office of Research and Development, U.S. Environmental Protection Agency, 109 TW Alexander Dr, Research Triangle Park, NC 27711, United States
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Pye H.O.T.,Ward-Caviness C.K.,Murphy B.N.,et al. Secondary organic aerosol association with cardiorespiratory disease mortality in the United States[J],2021,12(1).
APA Pye H.O.T.,Ward-Caviness C.K.,Murphy B.N.,Appel K.W.,&Seltzer K.M..(2021).Secondary organic aerosol association with cardiorespiratory disease mortality in the United States.Nature Communications,12(1).
MLA Pye H.O.T.,et al."Secondary organic aerosol association with cardiorespiratory disease mortality in the United States".Nature Communications 12.1(2021).
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