气候变化领域集成服务门户(CCPortal): Persistent CO2 photocatalysis for solar fuels in the dark

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DOI	10.1038/s41893-021-00681-y
	Persistent CO2 photocatalysis for solar fuels in the dark
	Loh J.Y.Y.; Kherani N.P.; Ozin G.A.
发表日期	2021
ISSN	2398-9629
起始页码	466
结束页码	473
卷号	4 期号:6
英文摘要	The hydrogenation of CO2 to hydrocarbon fuels via solar radiation offers a sustainable pathway towards a carbon-neutral energy cycle. However, the reaction is hindered by the intermittent availability of sunlight. This critical issue could be mitigated by engineering a materials system, known as persistent photocatalysis, that prolongs solar fuel production during overcast periods and into the evenings. During illumination, charge can be stored in a suitable capacitor or battery-like material that interfaces with the photocatalyst, while discharging occurs postillumination to continue driving the catalytic reaction. We discuss emerging trends and materials strategies to develop these catalyst systems and prolong the operation of photocatalysis. © 2021, Springer Nature Limited.
语种	英语
scopus关键词	Carbon dioxide; Photocatalysis; Catalyst system; Catalytic reactions; Critical issues; Emerging trends; Energy cycle; Hydrocarbon fuel; Materials systems; Solar fuels; Hydrogen fuels
来源期刊	Nature Sustainability
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/249787
作者单位	Electrical and Computer Engineering, University of Toronto, Toronto, ON, Canada; Materials Science and Engineering, University of Toronto, Toronto, ON, Canada; Department of Chemistry, University of Toronto, Toronto, ON, Canada
推荐引用方式 GB/T 7714	Loh J.Y.Y.,Kherani N.P.,Ozin G.A.. Persistent CO2 photocatalysis for solar fuels in the dark[J],2021,4(6).
APA	Loh J.Y.Y.,Kherani N.P.,&Ozin G.A..(2021).Persistent CO2 photocatalysis for solar fuels in the dark.Nature Sustainability,4(6).
MLA	Loh J.Y.Y.,et al."Persistent CO2 photocatalysis for solar fuels in the dark".Nature Sustainability 4.6(2021).