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DOI10.1016/j.atmosenv.2019.117069
Characteristics and provenance implications of rare earth elements and Sr–Nd isotopes in PM2.5 aerosols and PM2.5 fugitive dusts from an inland city of southeastern China
Yan Y.; Zheng Q.; Yu R.-L.; Hu G.-R.; Huang H.-B.; Lin C.-Q.; Cui J.-Y.; Yan Y.
发表日期2020
ISSN1352-2310
卷号220
英文摘要The chemical profiles of PM2.5 aerosols and PM2.5 fugitive dusts have been widely investigated in many cities; however, the characteristics and provenance implications of rare earth elements (REEs) and Sr–Nd isotopes have seldom been reported for PM2.5 aerosols and PM2.5 fugitive dusts. In this study, PM2.5 aerosol and PM2.5 fugitive (road, construction, and soil) dust samples were collected in Nanchang city, China, and analyzed for the characteristics and provenance implications via REEs and Sr–Nd isotopes. PM2.5 aerosol samples showed significantly higher ΣREE values (510.5 ± 347.4 mg kg−1) than PM2.5 fugitive dust samples (93.83 ± 35.23 mg kg−1 for road dust PM2.5, 185.0 ± 70.90 mg kg−1 for construction dust PM2.5, and 206.5 ± 34.28 mg kg−1 for soil dust PM2.5). Both the REE characteristic parameters and the chondrite-normalized REE distribution patterns indicated LREE enrichment and obvious negative Eu anomalies in both PM2.5 aerosol and fugitive dust samples. As shown in 87Sr/86Sr versus εNd(0) plot and ΣLREE/ΣHREE-Eu/Eu*-εNd(0) plot, the REEs in the PM2.5 fugitive dust samples were mainly affected by coal combustion, steelworks and construction cements and were also influenced by the background soil to some extent, while the REEs in the PM2.5 aerosol samples likely originated from both the investigated local sources and other nonlocal potential sources. © 2019 Elsevier Ltd
关键词Nanchang cityPM2.5Provenance compositionRare earth elementsSr–Nd isotope
语种英语
scopus关键词Aerosols; Coal combustion; Isotopes; Rare earth elements; Rare earths; Roads and streets; Soils; Chemical profiles; Distribution patterns; Nanchang city; Nd isotopes; Nonlocal potentials; PM2.5; Rare earth elements (REEs); Southeastern china; Coal dust; coal; lanthanide; neodymium; strontium; aerosol; chemical composition; dust; neodymium; neodymium isotope; particulate matter; pollutant source; rare earth element; strontium isotope; urban area; aerosol; Article; China; city; combustion; dust; particulate matter; priority journal; soil; suburban area; China; Jiangxi; Nanchang
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/249506
作者单位Department of Environmental Science and Engineering, Huaqiao University, Xiamen, 361021, China; Key Laboratory of Environmental Monitoring of University in Fujian Province, Xiamen, 361024, China; Analytical Laboratory of Beijing Research Institute of Uranium Geology, Beijing, 100029, China
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GB/T 7714
Yan Y.,Zheng Q.,Yu R.-L.,等. Characteristics and provenance implications of rare earth elements and Sr–Nd isotopes in PM2.5 aerosols and PM2.5 fugitive dusts from an inland city of southeastern China[J],2020,220.
APA Yan Y..,Zheng Q..,Yu R.-L..,Hu G.-R..,Huang H.-B..,...&Yan Y..(2020).Characteristics and provenance implications of rare earth elements and Sr–Nd isotopes in PM2.5 aerosols and PM2.5 fugitive dusts from an inland city of southeastern China.ATMOSPHERIC ENVIRONMENT,220.
MLA Yan Y.,et al."Characteristics and provenance implications of rare earth elements and Sr–Nd isotopes in PM2.5 aerosols and PM2.5 fugitive dusts from an inland city of southeastern China".ATMOSPHERIC ENVIRONMENT 220(2020).
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