气候变化领域集成服务门户(CCPortal): Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign

CCPortal

DOI	10.1016/j.atmosenv.2020.117384
	Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign
	Luo Y.; Dou K.; Fan G.; Huang S.; Si F.; Zhou H.; Wang Y.; Pei C.; Tang F.; Yang D.; Xi L.; Yang T.; Zhang T.; Liu W.
发表日期	2020
ISSN	1352-2310
卷号	226
英文摘要	As the development of megacities, combined air pollution has been of increasing concern in China, which is composed by primary pollution, such as Nitrogen dioxide (NO2), and the followed secondary pollution under certain meteorology circumstances and high concentration of precursors, such as tropospheric ozone, formaldehyde (HCHO) and fine particles. During PRIDE-GBA 2018 Campaign (Particles, Radicals, Intermediates from oxiDation of primary Emissions in Great Bay Area), we performed the high resolution vertical observations of pollution gases and aerosol, which are significant but scarce indexes in studying the mechanisms of tropospheric pollution, using remote sensing techniques. NO2 and HCHO column densities and vertical profiles are reconstructed from data of multi-axis differential optical absorption spectroscopy (MAX-DOAS). Tropospheric ozone profile and aerosol extinction are retrieved by the differential absorption light detection and ranging (LIDAR) system. In order to verifying the accuracy, we evaluated the consistency and reliability of MAX-DOAS and LIDAR measurements. The results showed reasonable agreement with in-situ and off-line observations at Canton Tower. A typical combined pollution process from Sep 29 to Oct 10 was analyzed in detail. More than 200 μg/m3 tropospheric ozone in this case was considered from the anthropogenic sources, including industry, power plant, residential and transportation. The high emission from local industry and polluted air transport from northeast brought the main precursors of this pollution process. The photochemical formation of tropospheric ozone was turned into a VOC-limited regime on polluted days. © 2020 Elsevier Ltd
关键词	Aerosol MAX-DOAS Precursor Tropospheric ozone Validation Vertical profile
语种	英语
scopus关键词	Absorption spectroscopy; Aerosols; Formaldehyde; Light absorption; Nitrogen oxides; Optical radar; Ozone; Photochemical forming; Reaction intermediates; Remote sensing; Troposphere; MAX-DOAS; Precursor; Tropospheric ozone; Validation; Vertical profile; Air pollution; formaldehyde; nitrogen dioxide; ozone; radical; volatile organic compound; aerosol; atmospheric pollution; formaldehyde; lidar; megacity; nitrogen dioxide; oxidation; ozone; remote sensing; troposphere; vertical distribution; absorption spectroscopy; aerosol; air pollution; air quality; Article; China; concentration (parameter); electric power plant; industrial area; light absorption; measurement accuracy; meteorology; oxidation; photochemistry; pollution monitoring; priority journal; reliability; remote sensing; residential area; traffic and transport
来源期刊	ATMOSPHERIC ENVIRONMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/249254
作者单位	Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, China; Institute for Environmental and Climate Research, Jinan University, Guangzhou, 510632, China; Guangzhou Environmental Monitoring Center, Guangzhou, 510060, China
推荐引用方式 GB/T 7714	Luo Y.,Dou K.,Fan G.,et al. Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign[J],2020,226.
APA	Luo Y..,Dou K..,Fan G..,Huang S..,Si F..,...&Liu W..(2020).Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign.ATMOSPHERIC ENVIRONMENT,226.
MLA	Luo Y.,et al."Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign".ATMOSPHERIC ENVIRONMENT 226(2020).