气候变化领域集成服务门户(CCPortal): A new anisotropic adaptive mesh photochemical model for ozone formation in power plant plumes

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DOI	10.1016/j.atmosenv.2020.117431
	A new anisotropic adaptive mesh photochemical model for ozone formation in power plant plumes
	Zheng J.; Fang F.; Wang Z.; Zhu J.; Li J.; Xiao H.; Pain C.C.
发表日期	2020
ISSN	1352-2310
卷号	229
英文摘要	In this work, an advanced dynamically adaptive unstructured mesh technique is introduced to photochemical modeling, which provides a consistent way to resolve the complex chemical transport processes over a wide range of spatial scales from meters (near point sources) up to hundred kilometers without the Gaussian distribution assumption (often used in existing subgrid Plume-in-Grid (PinG) models, such as RPM and SCICHEM). To assess the performance of the new photochemical model, the numerical results (NOx and O3) have been compared to the Southern Oxidants Study (SOS) 1999 aircraft plume measurements, where the range of the emission intensity is from 1.8 to 13.9 ton/h. The relative error in the peak value of NOx and O3 is between 10%–20% within 66 km downwind distance. The results show that the use of dynamically adaptive meshes can reproduce the details of the plume chemistry evolution: the slender puff structure of high NOx concentrations within a few kilometers width near the point sources, and the wing-like structure of ozone concentration during the plume growth, which is hard to capture for the PinG models or photochemical grid models. © 2020 Elsevier Ltd
关键词	Adaptive meshes CBM-Z Fluidity-Chem Ozone Photochemical model PinG Plume
语种	英语
scopus关键词	Mesh generation; Ozone; Adaptive meshes; Adaptive unstructured meshes; Aircraft plumes; Complex chemicals; Emission intensity; Numerical results; Ozone concentration; Photochemical modeling; Nitrogen oxides; nitrogen oxide; ozone; anisotropy; concentration (composition); numerical model; ozone; photochemistry; plume; power plant; advection; air quality; aircraft; anisotropy; Article; chemical model; chemical reaction; comparative study; computational fluid dynamics; concentration (parameter); controlled study; diffusion; eddy diffusivity; electric power plant; ozonation; photochemistry; plume; priority journal; simulation; troposphere; Neptunia
来源期刊	ATMOSPHERIC ENVIRONMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/249214
作者单位	Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, 361021, China; Department of Earth Science and Engineering, Imperial College London, Ireland; State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China; International Center for Climate and Environment Sciences, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
推荐引用方式 GB/T 7714	Zheng J.,Fang F.,Wang Z.,et al. A new anisotropic adaptive mesh photochemical model for ozone formation in power plant plumes[J],2020,229.
APA	Zheng J..,Fang F..,Wang Z..,Zhu J..,Li J..,...&Pain C.C..(2020).A new anisotropic adaptive mesh photochemical model for ozone formation in power plant plumes.ATMOSPHERIC ENVIRONMENT,229.
MLA	Zheng J.,et al."A new anisotropic adaptive mesh photochemical model for ozone formation in power plant plumes".ATMOSPHERIC ENVIRONMENT 229(2020).