气候变化领域集成服务门户(CCPortal): The calibration and deployment of a low-cost methane sensor

CCPortal

DOI	10.1016/j.atmosenv.2020.117440
	The calibration and deployment of a low-cost methane sensor
	Riddick S.N.; Mauzerall D.L.; Celia M.; Allen G.; Pitt J.; Kang M.; Riddick J.C.
发表日期	2020
ISSN	1352-2310
卷号	230
英文摘要	Since 1850 the atmospheric mixing ratio of methane (CH4), a potent greenhouse gas, has doubled. This increase is directly linked to an escalation in emissions from anthropogenic sources. An inexpensive means to identify and monitor CH4 emission sources and evaluate the efficacy of mitigation strategies is essential. However, sourcing reliable, low-cost, easy-to-calibrate sensors that are fit for purpose is challenging. A recent study showed that CH4 mixing ratio data from a low-power, low-cost CH4 sensor (Figaro TGS2600) agreed well with CH4 mixing ratios measured by a high precision sensor at mixing ratios between 1.85 ppm and 2 ppm. To investigate, as a proof of concept, if this low-cost sensor could be used to measure typical ambient CH4 mixing ratios, we operated a TGS2600 in conjunction with a Los Gatos Ultra-portable Greenhouse Gas Analyzer (UGGA) in controlled laboratory conditions. We then explored the sensor's long-term reliability by deploying the TGS2600 near an onshore gas terminal to calculate emissions from May to July 2018. Our initial studies showed that previously published linear algorithms could not convert TGS2600 output to CH4 mixing ratios measured by the UGGA. However, we derived a non-linear empirical relationship that could be used to reliably convert the output of a TGS2600 unit to CH4 mixing ratios over a range of 1.85–5.85 ppm that agree to a high-precision instrument output to ±0.01 ppm. Our study showed that the TGS2600 could be used to continuously measure variability in CH4 mixing ratios from 1.82 to 5.40 ppm for three months downwind of the gas terminal. Using a simplified Gaussian Plume approach, these mixing ratios correspond to an emission flux range of 0–238 g CH4 s−1, with average emission of 9.6 g CH4 s−1 from the currently active North Terminal and 1.6 g CH4 s−1 from the decommissioned South Terminal. Our work here demonstrates the feasibility of utilizing a low-cost sensor to detect methane leakage at concentrations close to ambient background levels, as long as the device is routinely calibrated with an accurate reference instrument. Having a widely deployed network of such low-cost CH4 sensors would allow improved identification, monitoring and mitigation of a variety of CH4 emissions. © 2020
关键词	Calibration Inexpensive Measurement Methane Mixing ratio
语种	英语
scopus关键词	Gas emissions; Greenhouse gases; Methane; Mixing; Anthropogenic sources; Atmospheric mixing; Controlled laboratories; Empirical relationships; Inexpensive means; Linear algorithms; Mitigation strategy; Reference instruments; Costs; alcohol; amide; butane; hydrogen; methane; natural gas; anthropogenic source; calibration; carbon emission; Gaussian method; greenhouse gas; methane; mitigation; mixing ratio; precision; sensor; strategic approach; air temperature; algorithm; Article; calibration; greenhouse gas; humidity; plume; priority journal; proof of concept; reliability; uncertainty; Galeus
来源期刊	ATMOSPHERIC ENVIRONMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/249176
作者单位	Department of Civil and Environmental Engineering, Princeton University, PrincetonNJ 08544, United States; Woodrow Wilson School of Public and International Affairs, Princeton University, PrincetonNJ 08544, United States; Centre for Atmospheric Science, University of Manchester, Manchester, M13 9PL, United Kingdom; Department of Civil Engineering and Applied Mechanics, McGill University, Montreal, H3A 0C3, Canada
推荐引用方式 GB/T 7714	Riddick S.N.,Mauzerall D.L.,Celia M.,et al. The calibration and deployment of a low-cost methane sensor[J],2020,230.
APA	Riddick S.N..,Mauzerall D.L..,Celia M..,Allen G..,Pitt J..,...&Riddick J.C..(2020).The calibration and deployment of a low-cost methane sensor.ATMOSPHERIC ENVIRONMENT,230.
MLA	Riddick S.N.,et al."The calibration and deployment of a low-cost methane sensor".ATMOSPHERIC ENVIRONMENT 230(2020).