气候变化领域集成服务门户(CCPortal): Differing effects of escalating pollution on absorption and scattering efficiencies of aerosols: Toward co-beneficial air quality enhancement and climate protection measures

CCPortal

DOI	10.1016/j.atmosenv.2020.117570
	Differing effects of escalating pollution on absorption and scattering efficiencies of aerosols: Toward co-beneficial air quality enhancement and climate protection measures
	Zhang Y.; Zhi G.; Jin W.; Wang L.; Guo S.; Shi R.; Sun J.; Cheng M.; Bi F.; Gao J.; Zhang B.; Wu J.; Shi Z.; Liu B.; Wang Z.; Li S.
发表日期	2020
ISSN	1352-2310
卷号	232
英文摘要	The mass absorption efficiency (MAE) and mass scattering efficiency (MSE) of aerosols are critical to their light extinction capacity. In winter in northern China, episodes of clear air and heavy haze alternately occur due to the high primary emission and secondary formation of aerosols, coupled with changing weather conditions. These occurrences facilitate detailed investigation of how significant changes in the pollution level impact the MAE and MSE, they also enable the determination of whether current air quality improvement measures are also beneficial to the mitigation of climate change, to avoid climatic side effects of attempts to clean the air. In the present study, a one-month observation campaign was conducted in Beijing, China, during the 2016–2017 winter season. A photoacoustic extinctiometer, which is an in situ measurement instrument, was used to investigate the aerosol absorption coefficient (σa) and scattering coefficient (σs) at an infra-red wavelength of 870 nm. The MAE and MSE were found to vary differently with increasing pollution level. A positive correlation between the particulate matter concentration (PM2.5) and the MAE was observed for PM2.5 < 100 μg m−3, with the increase in the MAE declining for PM2.5 = 100–200 μg m−3, and the MAE subsequently stabilizing. In contrast, the MSE continuously increased with increasing PM2.5. The single scattering albedo (SSA), which governs the climatic effect of aerosols, was observed to be a function of both σa and σs, increasing from 0.827 ± 0.018 (average ± standard deviation) for a bottom particulate matter concentration group of (0, 25] μg m−3 to 0.924 ± 0.007 for a top particulate matter concentration group of (300, 400] μg m−3, indicating a positive correlation between the SSA and PM2.5. These observations suggest a risk of current clean air measures weakening or eliminating the cooling effect of ambient aerosols in northern China. It seems that no previous study has involved the simultaneous acquisition of σa and σs at the same wavelength with the purpose of determining how increasing air pollution differently impacts the MAE and MSE. Practical measures that can be used to decrease the black carbon-to-PM2.5 ratio include phasing out or reducing black carbon-rich sources and promoting technologies that decrease the black carbon-to-organic carbon ratio. © 2020 Elsevier Ltd
关键词	Black carbon Mass absorption efficiency Mass scattering efficiency Optical property Single scattering albedo
语种	英语
scopus关键词	Aerosols; Air quality; Climate change; Efficiency; Light extinction; Organic carbon; Risk assessment; Absorption and scatterings; Air quality improvement; In-situ measurement; Mass scattering efficiency; Positive correlations; Scattering co-efficient; Simultaneous acquisition; Single scattering albedo; Particles (particulate matter); black carbon; organic carbon; absorption coefficient; absorption efficiency; adsorption; aerosol composition; air quality; albedo; atmospheric pollution; cooling; haze; in situ measurement; scattering; wavelength; absorption; aerosol; air pollution; air quality; Article; China; climate; climate change; climate warming; cooling; haze; humidity; light scattering; meteorology; optics; particle size; particulate matter; priority journal; radiative forcing; temperature; wind speed; winter; Beijing [China]; China
来源期刊	ATMOSPHERIC ENVIRONMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/249142
作者单位	College of Science, China University of Petroleum, Beijing, 102249, China; State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China; College of Chemistry and Chemical Engineering, Taiyuan University of Technology, Taiyuan, 030024, China; School of Physical Education, Shangrao Normal UniversityJiangxi 334001, China; College of Information Science and Engineering, Ocean University of China, Qingdao, 266100, China; Tangshan Institute of Environmental Protection, Tangshan, 063000, China; Department of Atmospheric Environment, Tangshan Bureau of Ecology and Environment, Tangshan, 301501, China; Hangu Administrative Zone Branch, Tangshan Bureau of Ecology and Environment, Tangshan, 301501, China; Liulin Branch, Lüliang Bureau of Ecology and Environment, Lüliang, 033300, China
推荐引用方式 GB/T 7714	Zhang Y.,Zhi G.,Jin W.,et al. Differing effects of escalating pollution on absorption and scattering efficiencies of aerosols: Toward co-beneficial air quality enhancement and climate protection measures[J],2020,232.
APA	Zhang Y..,Zhi G..,Jin W..,Wang L..,Guo S..,...&Li S..(2020).Differing effects of escalating pollution on absorption and scattering efficiencies of aerosols: Toward co-beneficial air quality enhancement and climate protection measures.ATMOSPHERIC ENVIRONMENT,232.
MLA	Zhang Y.,et al."Differing effects of escalating pollution on absorption and scattering efficiencies of aerosols: Toward co-beneficial air quality enhancement and climate protection measures".ATMOSPHERIC ENVIRONMENT 232(2020).