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DOI | 10.1016/j.atmosenv.2020.118090 |
Atmospheric fluxes of soluble nutrients and Fe: More than three years of wet and dry deposition measurements at Gran Canaria (Canary Islands) | |
López-García P.; Gelado-Caballero M.D.; Patey M.D.; Hernández-Brito J.J. | |
发表日期 | 2021 |
ISSN | 1352-2310 |
卷号 | 246 |
英文摘要 | Dust inputs to the oligotrophic waters of the subtropical North Atlantic are of significant importance to the biogeochemistry of the region. In this work, we present fluxes of particles, soluble elements (H+, major ions, Fe and organic ions) in dry deposition (DD) and wet deposition (WD) samples collected between September 2012 and April 2016. Positive Matrix Factorization Model (PMF) indicated four dominant factors influencing the elemental concentrations: marine, crustal and two anthropogenic. Soluble Fe fluxes appear to be affected predominantly by aerosol particle type, with higher values observed at lower dust loading. Although WD fluxes made up only a small fraction of total particle fluxes (12%), they represented an important input of soluble Fe and other nutrients such as nitrate (more than 50% of total amount deposited). This significant contribution to total deposition fluxes may have important consequences for primary production in the surface ocean. Mineral dust is the primary source of soluble atmospheric P to the north Atlantic, which is a region that is already P stressed. Our data show that DD dominates the total flux of soluble P to this area (∼87% of the total flux) and it may have a bigger impact in the diazotroph communities during the summer months when the water column is more stratified and nutrient inputs from deeper water are restricted. © 2020 Elsevier Ltd |
关键词 | AerosolDeposition fluxesDustEastern subtropical north atlanticSoluble ironSoluble nutrients |
语种 | 英语 |
scopus关键词 | Deposition; Dust; Factorization; Iron; Aerosol particles; Atmospheric fluxes; Deposition fluxes; Elemental concentrations; Nutrient inputs; Oligotrophic waters; Positive matrix factorization models; Primary production; Nutrients; acetic acid; ammonia; anion; bromide; calcium; chloride; fluoride; formic acid; iron; magnesium; nitrate; nitrite; oxalic acid; phosphate; potassium; sodium; sulfate; water; aerosol; anthropogenic effect; biogeochemistry; concentration (composition); dry deposition; dust; fractionation; iron; phosphorus; sampling; solubility; wet deposition; aerosol; atmosphere; autumn; biogeochemistry; boundary layer; Canary Islands; concentration process; controlled study; diazotroph; dry deposition; dust; marine environment; measurement accuracy; mineral dust; mineralogy; multivariate analysis; nutrient; particle size; positive matrix factorization model; priority journal; seasonal variation; summer; wet deposition; winter; Atlantic Ocean; Atlantic Ocean (North); Canary Islands; Gran Canaria; Las Palmas; Spain; Serinus canaria |
来源期刊 | ATMOSPHERIC ENVIRONMENT |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/248650 |
作者单位 | Chemistry Department, University of Las Palmas de Gran Canaria, Las Palmas de Gran Canaria, 35017, Spain; Ocean Technology and Engineering, National Oceanography Centre, Southampton, SO14 3ZH, United Kingdom; Oceanic Platform of the Canary Islands (PLOCAN), Carretera de Taliarte, Telde, 35214, Spain |
推荐引用方式 GB/T 7714 | López-García P.,Gelado-Caballero M.D.,Patey M.D.,et al. Atmospheric fluxes of soluble nutrients and Fe: More than three years of wet and dry deposition measurements at Gran Canaria (Canary Islands)[J],2021,246. |
APA | López-García P.,Gelado-Caballero M.D.,Patey M.D.,&Hernández-Brito J.J..(2021).Atmospheric fluxes of soluble nutrients and Fe: More than three years of wet and dry deposition measurements at Gran Canaria (Canary Islands).ATMOSPHERIC ENVIRONMENT,246. |
MLA | López-García P.,et al."Atmospheric fluxes of soluble nutrients and Fe: More than three years of wet and dry deposition measurements at Gran Canaria (Canary Islands)".ATMOSPHERIC ENVIRONMENT 246(2021). |
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