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DOI10.1016/j.atmosenv.2021.118225
Simulation of potential formation of atmospheric pollution from aboveground storage tank leakage after severe storms
Bi S.; Kiaghadi A.; Schulze B.C.; Bernier C.; Bedient P.B.; Padgett J.E.; Rifai H.; Griffin R.J.
发表日期2021
ISSN1352-2310
卷号248
英文摘要Damage by severe storms of infrastructure containing chemicals can cause widespread pollution of the atmosphere and nearby bodies of water. Because atmospheric monitoring equipment is inoperable in the periods after these storms, transport and fate modeling approaches are necessary to estimate the regional atmospheric concentrations of evaporated spill material and secondary pollutants from such events. Hypothetical spills from a single storage tank in Houston were used to evaluate the impact of different meteorological scenarios (Hurricanes Harvey in 2017 and Ike in 2008), leaked materials (oils and organic solvents), background chemical conditions, and cloud conditions on simulated air pollution. Due to differences in evaporation rate, downwind oil plumes are predicted to cover a broader region than organic solvent plumes, which remain concentrated along the path of the prevailing wind. Depending on assumptions regarding evaporation, mixing ratios of spilled material of up to 90 parts per million are predicted. Substantial formation of ozone (up to an enhancement of 130 parts per billion) and secondary organic aerosol (up to an enhancement of 30 μg m−3) could occur in the short-term aftermath of these storms within the downwind solvent plumes, with the magnitude dependent on the solar radiation, type of material, and background pollutant level. This highlights the potential vulnerability of residents and workers in downwind regions to evaporated spill materials and their degradation products. © 2021 Elsevier Ltd
关键词Evaporated spill materialsHurricaneOzoneSecondary organic aerosolTank leakage
语种英语
scopus关键词Atmospheric chemistry; Atmospheric movements; Degradation; Evaporation; Organic solvents; Storms; Tanks (containers); Water pollution; Water treatment; Aboveground storage tanks; Atmospheric concentration; Atmospheric monitoring; Atmospheric pollution; Chemical conditions; Degradation products; Parts per millions; Secondary organic aerosols; Air pollution; benzene; chemical compound; oil; organic solvent; ozone; solvent; toluene; aboveground biomass; atmospheric pollution; degradation; evaporation; leakage; oil spill; ozone; severe weather; solvent; storage tank; storm damage; vulnerability; air pollution; air quality; Article; chemical analysis; clinical evaluation; cloud; computer simulation; concentration process; dangerous goods; degradation kinetics; evaporation; hurricane; meteorology; plume; priority journal; secondary organic aerosol; simulation; solar radiation; storage; storage tank leakage; wind; wind speed; Houston; Texas; United States
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/248575
作者单位Department of Civil and Environmental Engineering, Rice University, Houston, TX 77005, United States; Department of Civil and Environmental Engineering, University of Houston, Houston, TX 77204, United States; Department of Chemical and Biomolecular Engineering, Rice University, Houston, TX 77005, United States
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Bi S.,Kiaghadi A.,Schulze B.C.,et al. Simulation of potential formation of atmospheric pollution from aboveground storage tank leakage after severe storms[J],2021,248.
APA Bi S..,Kiaghadi A..,Schulze B.C..,Bernier C..,Bedient P.B..,...&Griffin R.J..(2021).Simulation of potential formation of atmospheric pollution from aboveground storage tank leakage after severe storms.ATMOSPHERIC ENVIRONMENT,248.
MLA Bi S.,et al."Simulation of potential formation of atmospheric pollution from aboveground storage tank leakage after severe storms".ATMOSPHERIC ENVIRONMENT 248(2021).
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