气候变化领域集成服务门户(CCPortal): Long-range transport of Siberian biomass burning emissions to North America during FIREX-AQ

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DOI	10.1016/j.atmosenv.2021.118241
	Long-range transport of Siberian biomass burning emissions to North America during FIREX-AQ
	Johnson M.S.; Strawbridge K.; Knowland K.E.; Keller C.; Travis M.
发表日期	2021
ISSN	1352-2310
卷号	252
英文摘要	Biomass burning from wildfires is a significant global source of aerosol and trace gases which impact air quality, tropospheric and stratospheric composition, and climate. During the summer of 2019, wildfire activity in central and eastern Siberia occurred during the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign conducted in the United States between July 24 and September 6, 2019. Ground-based lidar observations from the Autonomous Mobile Ozone Lidar for Tropospheric Experiments (AMOLITE) system in Alberta, Canada retrieved frequent ozone (O3) and aerosol lamina in the free troposphere during the campaign. Simulated data from NASA's GEOS Composition Forecast (GEOS-CF) coupled chemistry meteorology model, TROPOspheric Monitoring Instrument (TROPOMI), and ground-based in situ measurements were applied to define the trans-Pacific and trans-Arctic transport pathways of Siberian biomass burning emissions resulting in the enhanced O3 and aerosol lamina observed by AMOLITE in western Canada. Siberian wildfires had some influence on North American air quality resulting in enhancements of surface carbon monoxide (CO) and fine particulate matter (PM2.5) concentrations in western Canada; however, minimal increases in surface-level O3 were measured as well as modeled by GEOS-CF. The impact in western Canada was larger in the free troposphere, demonstrated by GEOS-CF modeled and AMOLITE observed O3 lamina >20 ppb above background values and coincident model-predicted PM2.5 lamina >30 μg m−3. This study demonstrated that the Siberian biomass burning emissions in the summer of 2019 impacted tropospheric composition in western Canada, and potentially could have influenced areas in the vicinity of FIREX-AQ airborne and ground-based measurements in the United States, and should be considered in future studies. © 2021
关键词	Aerosol Air quality Biomass burning Chemical transport modeling Ozone Tropospheric composition
语种	英语
scopus关键词	Aerosols; Air quality; Biomass; Carbon monoxide; Fires; NASA; Optical radar; Troposphere; Biomass burning emissions; Biomass-burning; Chemical transport models; Eastern Siberia; Free troposphere; Global sources; Long range transport; PM$-2.5$; Trace gas; Tropospheric composition; Ozone; ammonia; black carbon; carbon monoxide; nitrate; organic carbon; ozone; sodium chloride; sulfate; aerosol; air quality; biomass burning; carbon monoxide; ground-based measurement; lidar; numerical model; particulate matter; trace gas; troposphere; aerosol; air quality; Article; biomass; biomass burning; Canada; chemical composition; concentration process; controlled study; exhaust gas; fire; fire influence on regional to global environment and air quality; forecasting; measurement accuracy; meteorology; North America; particulate matter 2.5; photochemistry; priority journal; public health campaign; remote sensing; secondary organic aerosol; simulation; spectroscopy; summer; surface area; troposphere; United States; wildfire; Alberta; Arctic; Canada; Canada; North America; Pacific Ocean; Siberia; United States; Alberta
来源期刊	ATMOSPHERIC ENVIRONMENT
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/248512
作者单位	Earth Science Division, NASA Ames Research Center, Moffett Field, CA, United States; Air Quality Processes Research Section, Environment and Climate Change Canada, Toronto, ON, Canada; Goddard Earth Science Technology and Research, Universities Space Research Association, Columbia, MD, United States; Global Modeling and Assimilation Office, NASA Goddard Space Flight Center, Greenbelt, MD, United States
推荐引用方式 GB/T 7714	Johnson M.S.,Strawbridge K.,Knowland K.E.,et al. Long-range transport of Siberian biomass burning emissions to North America during FIREX-AQ[J],2021,252.
APA	Johnson M.S.,Strawbridge K.,Knowland K.E.,Keller C.,&Travis M..(2021).Long-range transport of Siberian biomass burning emissions to North America during FIREX-AQ.ATMOSPHERIC ENVIRONMENT,252.
MLA	Johnson M.S.,et al."Long-range transport of Siberian biomass burning emissions to North America during FIREX-AQ".ATMOSPHERIC ENVIRONMENT 252(2021).