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DOI10.1016/j.atmosenv.2021.118569
Concentrations and size-distributions of water-soluble inorganic and organic species on aerosols over the Arctic Ocean observed during the US GEOTRACES Western Arctic Cruise GN01
Mukherjee P.; Marsay C.M.; Yu S.; Buck C.S.; Landing W.M.; Gao Y.
发表日期2021
ISSN1352-2310
卷号261
英文摘要Marine aerosols affect the climate directly and indirectly as well as serving as tracers of biogenic processes. Here we present the results from size-segregated and bulk aerosol samples collected from 2nd August to 10th October 2015 during the US GEOTRACES Arctic Ocean (GN01) expedition. Samples were analyzed for concentrations of major water-soluble organic and inorganic species, including acetate, formate, methanesulfonate (MSA), oxalate, propionate, chloride, nitrate, sulfate and major cations (Na+, K+, Mg2+, Ca2+, NH4+). Back-trajectory analysis was performed to categorize the wind patterns into three types; type 1, originating from the North Pacific and the Bering Sea, type–2, consisting entirely of marine Arctic air, and type 3, consisting of marine Arctic air mixed with air masses from the surrounding continents. Sea-salt was the major aerosol component, dominating in the coarse mode, 1.8–5.6 μm. Non-sea-salt sulfate and MSA were predominantly present in the fine mode, 0.18–0.32 μm, and MSA was associated with type 1 and type 2 air masses. The results from this study provide useful information on the origins and chemical processes involving these aerosol species over the Arctic in summer and help elucidate the significance of natural sources as contributors for the formation of cloud condensation nuclei. © 2021 Elsevier Ltd
关键词Arctic summer aerosolsFine mode MSA and Non-sea-salt-sulfateWater-soluble organic aerosols
语种英语
scopus关键词Chlorine compounds; Sulfur compounds; Volatile fatty acids; Air mass; Arctic ocean; Arctic summer aerosol; Concentration distributions; Fine mode methanesulphonate and non-sea-salt-sulphate; Inorganic species; Methanesulfonates; Sea salts; Sulphates; Water-soluble organic aerosol; Aerosols; acetic acid; ammonia; calcium ion; chloride; formic acid; inorganic compound; magnesium ion; mesylic acid; nitrate; organic compound; oxalic acid; propionic acid; sodium ion; sulfuric acid; aerosol; concentration (composition); condensation; size distribution; sulfate; wind power; aerosol; Arctic Ocean; Article; Bering Sea; chemical reaction; controlled study; water solubility; Arctic Ocean; Bering Sea; Pacific Ocean; Pacific Ocean (North)
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/248307
作者单位Department of Earth and Environmental Sciences, Rutgers University, Newark, NJ, United States; Skidaway Institute of Oceanography, University of Georgia, Savannah, GA, United States; Department of Marine and Coastal Sciences, Rutgers University, New Brunswick, NJ, United States; Department of Earth, Ocean and Atmospheric Science, Florida State University, Tallahassee, FL, United States
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Mukherjee P.,Marsay C.M.,Yu S.,et al. Concentrations and size-distributions of water-soluble inorganic and organic species on aerosols over the Arctic Ocean observed during the US GEOTRACES Western Arctic Cruise GN01[J],2021,261.
APA Mukherjee P.,Marsay C.M.,Yu S.,Buck C.S.,Landing W.M.,&Gao Y..(2021).Concentrations and size-distributions of water-soluble inorganic and organic species on aerosols over the Arctic Ocean observed during the US GEOTRACES Western Arctic Cruise GN01.ATMOSPHERIC ENVIRONMENT,261.
MLA Mukherjee P.,et al."Concentrations and size-distributions of water-soluble inorganic and organic species on aerosols over the Arctic Ocean observed during the US GEOTRACES Western Arctic Cruise GN01".ATMOSPHERIC ENVIRONMENT 261(2021).
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