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DOI10.1016/j.atmosenv.2021.118653
Vertical profile of aerosol characteristics including activation over a rain shadow region in India
Varghese M.; Jose J.; Anu A.S.; Konwar M.; Murugavel P.; Kalarikkal N.; Deshpande M.; Prabha T.V.
发表日期2021
ISSN1352-2310
卷号262
英文摘要Unique airborne observations of aerosol size spectral and chemical characteristics over the peninsular Indian region are illustrated in this case study. Multimodal lognormal distributions were required to fit the observed in situ aerosol size distribution. The aerosol composition and mixing state was deduced from the single-particle analyses of aerosols using the transmission electron microscope and soot photometer coupled with satellite retrieved aerosol classification, and back trajectory analyses. Organic carbon was the most prominent aerosol type found at all altitudes. Refractory black carbon aerosols which constituted about 10–12% of the aerosols in the boundary layer were primarily internally mixed with both inorganic and organic coating. Other major aerosol types were dust and sea salt, with the latter primarily found below 2 km. Further, the cloud forming ability of in-situ aerosols is tested through a cloud condensation nuclei closure analysis. The effective hygroscopicity decreased above cloud base due to the absence of sea salt aerosols. The change in large-scale winds with altitude affected the aerosol composition and hygroscopicity. The multimodal aerosol size distribution and hygroscopicity parameter (κ = 0.18) obtained for the cloud base aerosols over the rain shadow region are useful for studying aerosol-cloud interactions using regional cloud-resolving models. © 2021 Elsevier Ltd
关键词CAIPEEXCCN closureHygroscopicity parameterLognormal distributionSolapur
语种英语
scopus关键词Boundary layers; Codes (symbols); Organic carbon; Particle size analysis; Rain; Size distribution; Transmission electron microscopy; Aerosol composition; Aerosol size distributions; CAIPEEX; CCN closure; Hygroscopicity parameter; Log-normal distribution; Multi-modal; Rain shadow; Shadow regions; Solapur; Aerosols; aerosol; aerosol composition; airborne survey; black carbon; boundary layer; cloud condensation nucleus; particle size; rainfall; sea salt; vertical profile; India
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/248272
作者单位Indian Institute of Tropical Meteorology (Ministry of Earth Sciences), Dr. Homi Bhabha Road, Pashan, Pune, Maharashtra 411008, India; International and Inter University Centre for Nanoscience and Nanotechnology, Mahatma Gandhi University, Kottayam, Kerala 686560, India; School of Pure and Applied Physics, Mahatma Gandhi University, Kottayam, Kerala 686560, India; Department of Atmospheric and Space Science, Savitribai Phule Pune University, Ganeshkhind Road, Pune, Maharashtra 411007, India
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Varghese M.,Jose J.,Anu A.S.,et al. Vertical profile of aerosol characteristics including activation over a rain shadow region in India[J],2021,262.
APA Varghese M..,Jose J..,Anu A.S..,Konwar M..,Murugavel P..,...&Prabha T.V..(2021).Vertical profile of aerosol characteristics including activation over a rain shadow region in India.ATMOSPHERIC ENVIRONMENT,262.
MLA Varghese M.,et al."Vertical profile of aerosol characteristics including activation over a rain shadow region in India".ATMOSPHERIC ENVIRONMENT 262(2021).
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