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DOI | 10.1016/j.atmosenv.2021.118657 |
Simulation study on regional atmospheric oxidation capacity and precursor sensitivity | |
Li J.; An X.; Cui M.; Sun Z.; Wang C.; Li Y. | |
发表日期 | 2021 |
ISSN | 1352-2310 |
卷号 | 263 |
英文摘要 | In this study, an evaluation index of atmospheric oxidation capacity (AOIe) was established. A typical pollution event from October 3 to 8, 2015, and the WRF-Chem air quality model were used to simulate the distribution characteristics of atmospheric oxidation capacity (AOC) in Beijing and the influence of reducing emissions (NOx and VOCs) on regional AOC. The results showed that urban areas have stronger (approximately 11% higher on average) AOC than suburban areas. AOIe_G (the process of valence change in gaseous oxidants) contributed more to the regional AOC during the clean period. AOIe_G also contributed more in the daytime whereas AOIe_P (the process of valence change in particulate state) contributed more at nighttime, with the highest contribution accounting for 72% and 69%, and the corresponding peak concentrations appearing at 14:00 and 06:00, respectively. In addition, compared with NOx reduction, the effect of reducing VOCs on reducing AOC was more significant. © 2021 Elsevier Ltd |
关键词 | Evaluation index of AOC (AOIe)NOxSensitivity of ozone precursorVOCsWRF-Chem model |
语种 | 英语 |
scopus关键词 | Air quality; Oxidation; Air quality modelling; Atmospheric oxidation capacity; Evaluation index; Evaluation index of atmospheric oxidation capacity (AOIe); Oxidation precursors; Sensitivity of ozone precursor; Simulation studies; Valence change; WRF-chem model; WRF/Chem; Nitrogen oxides; air quality; atmospheric pollution; concentration (composition); nitric oxide; oxidant; oxidation; sensitivity analysis; simulation; volatile organic compound |
来源期刊 | ATMOSPHERIC ENVIRONMENT
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/248255 |
作者单位 | Institute of Atmospheric Composition and Environmental Meteorology, CAMS, Chinese Academy of Meteorological Sciences, Beijing, 100081, China; 78127 Unit of the Chinese People's Liberation Army, Chengdu, 610000, China; Institute of Urban Meteorology, China Meteorological Administration, Beijing, 100089, China |
推荐引用方式 GB/T 7714 | Li J.,An X.,Cui M.,et al. Simulation study on regional atmospheric oxidation capacity and precursor sensitivity[J],2021,263. |
APA | Li J.,An X.,Cui M.,Sun Z.,Wang C.,&Li Y..(2021).Simulation study on regional atmospheric oxidation capacity and precursor sensitivity.ATMOSPHERIC ENVIRONMENT,263. |
MLA | Li J.,et al."Simulation study on regional atmospheric oxidation capacity and precursor sensitivity".ATMOSPHERIC ENVIRONMENT 263(2021). |
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