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DOI10.1016/j.atmosenv.2021.118748
Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region
Ahn S.H.; Yoon Y.J.; Choi T.J.; Lee J.Y.; Kim Y.P.; Lee B.Y.; Ritter C.; Aas W.; Krejci R.; Ström J.; Tunved P.; Jung C.H.
发表日期2021
ISSN1352-2310
卷号267
英文摘要To determine the direct and indirect effects of aerosols on climate, it is important to know the spatial and temporal variations in cloud condensation nuclei (CCN) concentrations. Although many types of CCN measurements are available, extensive CCN measurements are challenging because of the complexity and high operating cost, especially in remote areas. As aerosol optical depth (AOD) can be readily observed by remote sensing, many attempts have been made to estimate CCN concentrations from AOD. In this study, the CCN–AOD relationship is parameterized based on CCN ground measurements from the Zeppelin Observatory (78.91° N, 11.89° E, 474 m asl) in the Arctic region. The AOD measurements were obtained from the Ny-Ålesund site (78.923° N, 11.928° E) and Modern-Era Retrospective Analysis for Research and Applications, Version 2 reanalysis. Our results show a CCN–AOD correlation with a coefficient of determination R2 of 0.59. Three additional estimation models for CCN were presented based on the following data: (i) in situ aerosol chemical composition, (ii) in situ aerosol optical properties, and (iii) chemical composition of AOD obtained from reanalysis data. The results from the model using in situ aerosol optical properties reproduced the observed CCN concentration most efficiently, suggesting that the contribution of BC to CCN concentration should be considered along with that of sulfate. © 2021 Elsevier Ltd
关键词Aerosol optical depthArctic regionBlack carbonCCN–AOD relationshipCloud condensation nuclei
语种英语
scopus关键词Aerosols; Carbon; Optical properties; Remote sensing; Sulfur compounds; Aerosol optical depths; Aerosol optical property; Arctic regions; Black carbon; Cloud condensation nuclei; Cloud condensation nucleus–aerosol optical depth relationship; Indirect effects; Reanalysis; Condensation; black carbon; sulfate; aerosol; cloud condensation nucleus; concentration (composition); optical depth; optical property; remote sensing; aerosol; air temperature; Arctic; Article; autumn; boundary layer; chemical composition; cloud; cloud condensation nuclei; comparative study; concentration (parameter); environmental parameters; light absorption; light scattering; measurement; optical depth; particle size; photometry; remote sensing; seasonal variation; secondary organic aerosol; spring; time series analysis; troposphere; wettability; winter; Arctic
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/248183
作者单位Korea Polar Research Institute (KOPRI), 26 Songdomirae-ro, Yeonsu-gu, Incheon, 21990, South Korea; University of Science and Technology, 217 Gajeong-ro, Yuseong-gu, Daejeon, 34113, South Korea; Department of Environmental Science and Engineering, Ewha Womans University, Seoul, 03760, South Korea; Department of Chemical Engineering and Materials Science, Ewha Womans University, Seoul, 03760, South Korea; Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung, Telegrafenberg A45, Potsdam, 14473, Germany; NILU – Norwegian Institute for Air Research, Kjeller, 2027, Norway; Department of Environmental Science & Bolin Centre for Climate Research, Stockholm University, Stockholm, S 106 91, Sweden; Department of Health Management, Kyungin Women's University, Incheon, 21041, South Korea
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Ahn S.H.,Yoon Y.J.,Choi T.J.,et al. Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region[J],2021,267.
APA Ahn S.H..,Yoon Y.J..,Choi T.J..,Lee J.Y..,Kim Y.P..,...&Jung C.H..(2021).Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region.ATMOSPHERIC ENVIRONMENT,267.
MLA Ahn S.H.,et al."Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region".ATMOSPHERIC ENVIRONMENT 267(2021).
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