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DOI10.1016/j.atmosenv.2021.118806
Long-range transport of La Soufrière volcanic plume to the western North Pacific: Influence on atmospheric mercury and aerosol properties
Ravindra Babu S.; Nguyen L.S.P.; Sheu G.-R.; Griffith S.M.; Pani S.K.; Huang H.-Y.; Lin N.-H.
发表日期2022
ISSN1352-2310
卷号268
英文摘要Volcanic eruptions are important natural sources of gases and aerosols to the environment. However, their impact on the global cycle of trace elements, including mercury (Hg), remains poorly understood. On 9 April 2021, La Soufrière volcano (13.33°N, 61.18°W) erupted in the Caribbean Sea. Ozone Monitoring Instrument (OMI) measurements of sulfur dioxide (SO2) tracked the transport of volcanic SO2 in the troposphere over long distances from the source, including to the western North Pacific ∼10 day after eruption. A spike in gaseous and particle-bound mercury concentrations along with a peak in aerosol back-scattering coefficient at Lulin Atmospheric Background Station (LABS, 23.47°N, 120.87°E; 2862 m AMSL) coincided with the volcanic plume transport on 19 April. The slope of gaseous elemental mercury vs. carbon monoxide concentrations during the event was 0.027, which is distinctly higher than for Southeast Asia biomass burning (slope = 0.005) and East Asia outflow (0.011) pollution sources. Arrival of the plume high above Taiwan was confirmed by significant changes in signature aerosol properties. Thus, with critical observational evidence, our study reported for the first time enhanced mercury levels ∼18000 km downwind from a volcano source, providing an important check on volcanic Hg emission strength. © 2021
关键词La Soufrière volcanoLong-range transportLulin atmospheric background stationMercury
语种英语
scopus关键词Aerosols; Atmospheric movements; Backscattering; Carbon monoxide; Lanthanum; Lanthanum compounds; Mercury compounds; Sulfur dioxide; Trace elements; Aerosol properties; Atmospheric mercury; La soufriere volcano; Long range transport; Lulin atmospheric background station; Mercury; Volcanic eruptions; Volcanic plume; Volcanics; Western North Pacific; Volcanoes; carbon monoxide; mercury; ozone; sulfate; sulfur dioxide; aerosol; biomass burning; carbon monoxide; concentration (composition); mercury (element); outflow; plume; sulfur dioxide; trace element; troposphere; volcanic eruption; aerosol; air pollution; airborne particle; albedo; altitude; Article; atmospheric dispersion; biomass production; chemical modification; concentration (parameter); depolarization; dust; gas; geographic mapping; light absorption; light scattering; limit of detection; optical depth; oxidation; particle size; particulate matter 2.5; plume; pollution monitoring; pollution transport; refraction index; stratosphere; time series analysis; troposphere; volcanic ash; Pacific Ocean; Pacific Ocean (North); Southeast Asia; Taiwan
来源期刊ATMOSPHERIC ENVIRONMENT
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/248162
作者单位Department of Atmospheric Sciences, National Central University, Taoyuan, 32001, Taiwan; Center for Environmental Monitoring and Technology, National Central University, Taoyuan, 32001, Taiwan; Faculty of Environment, VNUHCM-University of Science, Vietnam National University, Ho Chi Minh City, Viet Nam
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Ravindra Babu S.,Nguyen L.S.P.,Sheu G.-R.,et al. Long-range transport of La Soufrière volcanic plume to the western North Pacific: Influence on atmospheric mercury and aerosol properties[J],2022,268.
APA Ravindra Babu S..,Nguyen L.S.P..,Sheu G.-R..,Griffith S.M..,Pani S.K..,...&Lin N.-H..(2022).Long-range transport of La Soufrière volcanic plume to the western North Pacific: Influence on atmospheric mercury and aerosol properties.ATMOSPHERIC ENVIRONMENT,268.
MLA Ravindra Babu S.,et al."Long-range transport of La Soufrière volcanic plume to the western North Pacific: Influence on atmospheric mercury and aerosol properties".ATMOSPHERIC ENVIRONMENT 268(2022).
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