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DOI10.5194/acp-20-8593-2020
Airborne in situ measurements of aerosol size distributions and black carbon across the Indo-Gangetic Plain during SWAAMI-RAWEX
Gogoi M.M.; Jayachandran V.N.; Vaishya A.; Babu S.N.S.; Satheesh S.K.; Moorthy K.K.
发表日期2020
ISSN1680-7316
起始页码8593
结束页码8610
卷号20期号:14
英文摘要During the combined South-West Asian Aerosol-Monsoon Interactions and Regional Aerosol Warming Experiment (SWAAMI-RAWEX), collocated airborne measurements of aerosol number-size distributions in the size (diameter) regime 0.5 to 20 μ m and black carbon (BC) mass concentrations were made across the Indo-Gangetic Plain (IGP), for the first time, from three distinct locations, just prior to the onset of the Indian summer monsoon. These measurements provided an east-west transect of region-specific properties of aerosols as the environment transformed from mostly arid conditions of the western IGP (represented by Jodhpur, JDR) having dominance of natural aerosols to the central IGP (represented by Varanasi, VNS) having very high anthropogenic emissions, to the eastern IGP (represented by the coastal station Bhubaneswar, BBR) characterized by a mixture of the IGP outflow and marine aerosols. Despite these, the aerosol size distribution revealed an increase in coarse mode concentration and coarse mode mass fraction (fractional contribution to the total aerosol mass) with the increase in altitude across the entire IGP, especially above the well-mixed region. Consequently, both the mode radii and geometric mean radii of the size distributions showed an increase with altitude. However, near the surface and within the atmospheric boundary layer (ABL), the features were specific to the different subregions, with the highest coarse mode mass fraction (FMC ∼ 72 %) in the western IGP and highest accumulation fraction in the central IGP with the eastern IGP in between. The elevated coarse mode fraction is attributed to mineral dust load arising from local production as well as due to advection from the west. This was further corroborated by data from the Cloud-Aerosol Transport System (CATS) on board the International Space Station (ISS), which also revealed that the vertical extent of dust aerosols reached as high as 5 km during this period. Mass concentrations of BC were moderate (∼ 1 μ g m-3) with very little altitude variation up to 3.5 km, except over VNS where very high concentrations were seen near the surface and within the ABL. The BC-induced atmospheric heating rate was highest near the surface at VNS (∼ 0:81 K d-1), while showing an increasing pattern with altitude at BBR (∼ 0:35 K d-1 at the ceiling altitude). © 2020 Author(s).
语种英语
scopus关键词accumulation; aerosol; airborne survey; black carbon; boundary layer; dust; experimental study; in situ measurement; size distribution; Gangetic Plain
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/247635
作者单位Space Physics Laboratory, Vikram Sarabhai Space Centre, Thiruvananthapuram, 695022, India; School of Arts and Sciences, Global Centre for Environment and Energy, Ahmedabad University, Ahmedabad, 380009, India; Centre for Atmospheric and Oceanic Sciences, Indian Institute of Science, Bengaluru, 560012, India; Divecha Centre for Climate Change, Indian Institute of Science, Bengaluru, 560012, India
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Gogoi M.M.,Jayachandran V.N.,Vaishya A.,et al. Airborne in situ measurements of aerosol size distributions and black carbon across the Indo-Gangetic Plain during SWAAMI-RAWEX[J],2020,20(14).
APA Gogoi M.M.,Jayachandran V.N.,Vaishya A.,Babu S.N.S.,Satheesh S.K.,&Moorthy K.K..(2020).Airborne in situ measurements of aerosol size distributions and black carbon across the Indo-Gangetic Plain during SWAAMI-RAWEX.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(14).
MLA Gogoi M.M.,et al."Airborne in situ measurements of aerosol size distributions and black carbon across the Indo-Gangetic Plain during SWAAMI-RAWEX".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.14(2020).
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