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DOI10.5194/acp-20-10063-2020
The value of remote marine aerosol measurements for constraining radiative forcing uncertainty
Regayre L.A.; Schmale J.; Johnson J.S.; Tatzelt C.; Baccarini A.; Henning S.; Yoshioka M.; Stratmann F.; Gysel-Beer M.; Grosvenor D.P.; Carslaw K.S.
发表日期2020
ISSN1680-7316
起始页码10063
结束页码10072
卷号20期号:16
英文摘要Aerosol measurements over the Southern Ocean are used to constrain aerosol-cloud interaction radiative forcing (RFaci) uncertainty in a global climate model. Forcing uncertainty is quantified using 1 million climate model variants that sample the uncertainty in nearly 30 model parameters. Measurements of cloud condensation nuclei and other aerosol properties from an Antarctic circumnavigation expedition strongly constrain natural aerosol emissions: default sea spray emissions need to be increased by around a factor of 3 to be consistent with measurements. Forcing uncertainty is reduced by around 7% using this set of several hundred measurements, which is comparable to the 8% reduction achieved using a diverse and extensive set of over 9000 predominantly Northern Hemisphere measurements. When Southern Ocean and Northern Hemisphere measurements are combined, uncertainty in RFaci is reduced by 21 %, and the strongest 20% of forcing values are ruled out as implausible. In this combined constraint, observationally plausible RFaci is around 0.17Wm-2 weaker (less negative) with 95% credible values ranging from-2:51 to-1:17Wm-2 (standard deviation of-2:18 to-1:46Wm-2). The Southern Ocean and Northern Hemisphere measurement datasets are complementary because they constrain different processes. These results highlight the value of remote marine aerosol measurements. © 2020 Laser Institute of America. All rights reserved.
语种英语
scopus关键词aerosol; climate modeling; cloud condensation nucleus; cloud radiative forcing; global climate; Northern Hemisphere; uncertainty analysis; Southern Ocean
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/247555
作者单位Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2g9JT, United Kingdom; Paul Scherrer Institute, Laboratory of Atmospheric Chemistry, Villigen, Switzerland; École Polytechnique Fédéderale de Lausanne, Lausanne, Switzerland; Leibniz Institute for Tropospheric Research, Leipzig, Germany; National Centre for Atmospheric Science, Leeds, United Kingdom
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Regayre L.A.,Schmale J.,Johnson J.S.,et al. The value of remote marine aerosol measurements for constraining radiative forcing uncertainty[J],2020,20(16).
APA Regayre L.A..,Schmale J..,Johnson J.S..,Tatzelt C..,Baccarini A..,...&Carslaw K.S..(2020).The value of remote marine aerosol measurements for constraining radiative forcing uncertainty.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(16).
MLA Regayre L.A.,et al."The value of remote marine aerosol measurements for constraining radiative forcing uncertainty".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.16(2020).
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