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DOI10.5194/acp-20-13611-2020
On mineral dust aerosol hygroscopicity
Chen L.; Peng C.; Gu W.; Fu H.; Jian X.; Zhang H.; Zhang G.; Zhu J.; Wang X.; Tang M.
发表日期2020
ISSN1680-7316
起始页码13611
结束页码13626
卷号20期号:21
英文摘要Despite its importance, hygroscopicity of mineral dust aerosol remains highly uncertain. In this work, we investigated water adsorption and hygroscopicity of different mineral dust samples at 25 °C, via measurement of sample mass at different relative humidity (RH, up to 90 %) using a vapor sorption analyzer. Mineral dust samples examined (21 in total) included seven authentic mineral dust samples from different regions in the world and 14 major minerals contained in mineral dust aerosol. At 90%RH, the mass ratios of adsorbed water to the dry mineral ranged from 0.0011 to 0.3080, largely depending on the BET surface areas of mineral dust samples. The fractional surface coverages of adsorbed water were determined to vary between 1.26 and 8.63 at 90%RH, and it was found that the Frenkel-Halsey-Hill (FHH) adsorption isotherm could describe surface coverages of adsorbed water as a function of RH well, with AFHH and BFHH parameters in the range of 0.15-4.39 and 1.10-1.91, respectively. The comprehensive and robust data obtained would largely improve our knowledge of hygroscopicity of mineral dust aerosol. © Author(s) 2020.
语种英语
scopus关键词aerosol composition; aerosol formation; dust; hygroscopicity; mineral dust; relative humidity
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/247374
作者单位State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, China; State Key Laboratory of Marine Environmental Science, College of Ocean and Earth Sciences, Xiamen University, Xiamen, China; CAS Key Laboratory of Mineralogy and Metallogeny, Guangdong Provincial Key Laboratory of Mineral Physics and Material Research and Development, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, China; University of Chinese Academy of Sciences, Beijing, China; Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
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GB/T 7714
Chen L.,Peng C.,Gu W.,et al. On mineral dust aerosol hygroscopicity[J],2020,20(21).
APA Chen L..,Peng C..,Gu W..,Fu H..,Jian X..,...&Tang M..(2020).On mineral dust aerosol hygroscopicity.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(21).
MLA Chen L.,et al."On mineral dust aerosol hygroscopicity".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.21(2020).
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