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DOI | 10.5194/acp-21-915-2021 |
Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM2.5 control in Beijing | |
Wang Y.; Li Z.; Wang Q.; Jin X.; Yan P.; Cribb M.; Li Y.; Yuan C.; Wu H.; Wu T.; Ren R.; Cai Z. | |
发表日期 | 2021 |
ISSN | 1680-7316 |
起始页码 | 915 |
结束页码 | 926 |
卷号 | 21期号:2 |
英文摘要 | A comprehensive field experiment measuring aerosol chemical and physical properties at a suburban site in Beijing around the 2019 Spring Festival was carried out to investigate the impact of reduced anthropogenic emissions on aerosol formation. Sharply reduced sulfur dioxide (SO2) and nitrogen dioxide (NO2) concentrations during the festival holiday resulted in an unexpected increase in the surface ozone (O3) concentration caused by the strong O3- titration phenomenon. Simultaneously, the reduced anthropogenic emissions resulted in massive decreases in particle number concentration at all sizes and the mass concentrations of organics and black carbon. However, the mass concentrations of inorganics (especially sulfate) decreased weakly. Detailed analyses of the sulfur oxidation ratio and the nitrogen oxidation ratio suggest that sulfate formation during the holiday could be promoted by enhanced nocturnal aqueousphase chemical reactions between SO2 and O3 under moderate relative humidity (RH) conditions (40% |
语种 | 英语 |
scopus关键词 | aerosol formation; anthropogenic source; atmospheric pollution; concentration (composition); emission; festival; nitrogen dioxide; ozone; particulate matter; physicochemical property; sulfur dioxide; Beijing [Beijing (ADS)]; Beijing [China]; China; Hebei; Tianjin |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/247208 |
作者单位 | Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing, 210044, China; State Key Laboratory of Remote Sensing Science, Beijing Normal University, Beijing, 100875, China; Earth System Science Interdisciplinary Center, Department of Atmospheric and Oceanic Science, University of Maryland, College Park, MD, United States; CMA Meteorological Observation Center, Centre for Atmosphere Watch and Services, Beijing, 100081, China |
推荐引用方式 GB/T 7714 | Wang Y.,Li Z.,Wang Q.,et al. Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM2.5 control in Beijing[J],2021,21(2). |
APA | Wang Y..,Li Z..,Wang Q..,Jin X..,Yan P..,...&Cai Z..(2021).Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM2.5 control in Beijing.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(2). |
MLA | Wang Y.,et al."Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM2.5 control in Beijing".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.2(2021). |
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