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DOI | 10.5194/acp-21-5705-2021 |
A study of the effect of aerosols on surface ozone through meteorology feedbacks over China | |
Qu Y.; Voulgarakis A.; Wang T.![]() | |
发表日期 | 2021 |
ISSN | 1680-7316 |
起始页码 | 5705 |
结束页码 | 5718 |
卷号 | 21期号:7 |
英文摘要 | Interactions between aerosols and gases in the atmosphere have been the focus of an increasing number of studies in recent years. Here, we focus on aerosol effects on tropospheric ozone that involve meteorological feedbacks induced by aerosol-radiation interactions. Specifically, we study the effects that involve aerosol influences on the transport of gaseous pollutants and on atmospheric moisture, both of which can impact ozone chemistry. For this purpose, we use the UK Earth System Model (UKESM1), with which we performed sensitivity simulations including and excluding the aerosol direct radiative effect (ADE) on atmospheric chemistry, and focused our analysis on an area with a high aerosol presence, namely China. By comparing the simulations, we found that ADE reduced shortwave radiation by 11 % in China and consequently led to lower turbulent kinetic energy, weaker horizontal winds and a shallower boundary layer (with a maximum of 102.28 m reduction in north China). On the one hand, the suppressed boundary layer limited the export and diffusion of pollutants and increased the concentration of CO, SO2, NO, NO2, PM2.5 and PM10 in the aerosol-rich regions. The |
语种 | 英语 |
scopus关键词 | aerosol; atmospheric chemistry; atmospheric gas; boundary layer; climate feedback; concentration (composition); meteorology; model test; ozone; radiative forcing; shortwave radiation; troposphere; wind field; China |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/246975 |
作者单位 | School of Atmospheric Sciences, Nanjing University, Nanjing, China; Leverhulme Centre for Wildfires, Environment and Society, Department of Physics, Imperial College London, London, United Kingdom; School of Intelligent Science and Control Engineering, Jinling Institute of Technology, Nanjing, China; School of Environmental Engineering, Technical University of Crete, Crete, Greece; School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing, China |
推荐引用方式 GB/T 7714 | Qu Y.,Voulgarakis A.,Wang T.,et al. A study of the effect of aerosols on surface ozone through meteorology feedbacks over China[J],2021,21(7). |
APA | Qu Y..,Voulgarakis A..,Wang T..,Kasoar M..,Wells C..,...&Mansfield L..(2021).A study of the effect of aerosols on surface ozone through meteorology feedbacks over China.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(7). |
MLA | Qu Y.,et al."A study of the effect of aerosols on surface ozone through meteorology feedbacks over China".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.7(2021). |
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