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DOI10.5194/acp-21-12613-2021
Measurement report: Biogenic volatile organic compound emission profiles of rapeseed leaf litter and its secondary organic aerosol formation potential
Abis L.; Kalalian C.; Lunardelli B.; Wang T.; Zhang L.; Chen J.; Perrier S.; Loubet B.; Ciuraru R.; George C.
发表日期2021
ISSN1680-7316
起始页码12613
结束页码12629
卷号21期号:16
英文摘要We analysed the biogenic volatile organic compound (BVOC) emissions from rapeseed leaf litter and their potential to create secondary organic aerosols (SOAs) under three different conditions, i.e., (i) in the presence of UV light irradiation, (ii) in the presence of ozone, and (iii) with both ozone and UV light. These experiments were performed in a controlled atmospheric simulation chamber containing leaf litter samples, where BVOC and aerosol number concentrations were measured for 6 d. Our results show that BVOC emission profiles were affected by UV light irradiation which increased the summed BVOC emissions compared to the experiment with solely O3. Furthermore, the diversity of emitted VOCs from the rapeseed litter also increased in the presence of UV light irradiation. SOA formation was observed when leaf litter was exposed to both UV light and O3, indicating a potential contribution to particle formation or growth at local scales. To our knowledge, this study investigates, for the first time, the effect of UV irradiation and O3 exposure on both VOC emissions and SOA formation for leaf litter samples. A detailed discussion about the processes behind the biological production of the most important VOC is proposed. © 2021 The Author(s).
语种英语
scopus关键词aerosol; computer simulation; concentration (composition); leaf litter; numerical model; ultraviolet radiation; volatile organic compound; Brassica napus
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/246634
作者单位Univ Lyon, Université Claude Bernard Lyon 1, CNRS, IRCELYON, Villeurbanne, 69626, France; Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai, 200433, China; INRAE, UMR ECOSYS, AgroParisTech, Université Paris-Saclay, Thiverval-Grignon, 78850, France; Technische Universität Berlin, Umweltchemie und Luftrinhaltunz, Straße des 17. Juni 135, Berlin, 10623, Germany
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Abis L.,Kalalian C.,Lunardelli B.,et al. Measurement report: Biogenic volatile organic compound emission profiles of rapeseed leaf litter and its secondary organic aerosol formation potential[J],2021,21(16).
APA Abis L..,Kalalian C..,Lunardelli B..,Wang T..,Zhang L..,...&George C..(2021).Measurement report: Biogenic volatile organic compound emission profiles of rapeseed leaf litter and its secondary organic aerosol formation potential.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(16).
MLA Abis L.,et al."Measurement report: Biogenic volatile organic compound emission profiles of rapeseed leaf litter and its secondary organic aerosol formation potential".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.16(2021).
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