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DOI10.5194/acp-21-13011-2021
Opinion: The germicidal effect of ambient air (open-air factor) revisited
Anthony Cox R.; Ammann M.; Crowley J.N.; Griffiths P.T.; Herrmann H.; Hoffmann E.H.; Jenkin M.E.; Faye McNeill V.; Mellouki A.; Penkett C.J.; Tilgner A.; Wallington T.J.
发表日期2021
ISSN1680-7316
起始页码13011
结束页码13018
卷号21期号:17
英文摘要The term open-air factor (OAF) was coined following microbiological research in the 1960s and 1970s which established that rural air had powerful germicidal properties and attributed this to Criegee intermediates formed in the reaction of ozone with alkenes. We have re-evaluated those early experiments applying the current state of knowledge of ozone-alkene reactions. Contrary to previous speculation, neither Criegee intermediates nor the HO radicals formed in their decomposition are directly responsible for the germicidal activity attributed to the OAF. We identify other potential candidates, which are formed in ozone-alkene reactions and have known (and likely) germicidal properties, but the compounds responsible for the OAF remain a mystery. There has been very little research into the OAF since the 1970s, and this effect seems to have been largely forgotten. In this opinion piece we remind the community of the germicidal open-air factor. Given the current global pandemic spread by an airborne pathogen, understanding the natural germicidal effects of ambient air, solving the mystery of the open-air factor and determining how this effect can be used to improve human welfare should be a high priority for the atmospheric science community. © 2021 The Author(s).
语种英语
scopus关键词aerobiology; air quality; alkene; ambient air; atmospheric pollution; epidemic; germ cell; ozone
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/246614
作者单位Centre for Atmospheric Science, Department of Chemistry, University of Cambridge, Cambridge, CB2 1EP, United Kingdom; Laboratory of Environmental Chemistry, Paul Scherrer Institut, Villigen, 5232, Switzerland; Division of Atmospheric Chemistry, Max Planck Institute for Chemistry, Mainz, 55128, Germany; National Centre for Atmospheric Science, Department of Chemistry, Cambridge University, Cambridge, CB21EW, United Kingdom; Atmospheric Chemistry Department (ACD), Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, 04318, Germany; Atmospheric Chemistry Services, Okehampton, EX20 4QB, United Kingdom; Department of Chemical Engineering, Columbia University, New York, NY 10027, United States; ICARE-CNRS, Orléans Cedex 2, 45071, France; NIHR BioResource for Translational Research, University of Cambridge, Hills Road, Cambridge, CB2 0QQ, United Kingdom; Ford Motor Company, Research and Advanced Engineering, Dearborn, MI 48121-2053, United States
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GB/T 7714
Anthony Cox R.,Ammann M.,Crowley J.N.,et al. Opinion: The germicidal effect of ambient air (open-air factor) revisited[J],2021,21(17).
APA Anthony Cox R..,Ammann M..,Crowley J.N..,Griffiths P.T..,Herrmann H..,...&Wallington T.J..(2021).Opinion: The germicidal effect of ambient air (open-air factor) revisited.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(17).
MLA Anthony Cox R.,et al."Opinion: The germicidal effect of ambient air (open-air factor) revisited".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.17(2021).
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