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DOI10.1126/science.1254509
Formation temperatures of thermogenic and biogenic methane
Stolper D.A.; Lawson M.; Davis C.L.; Ferreira A.A.; Santos Neto E.V.; Ellis G.S.; Lewan M.D.; Martini A.M.; Tang Y.; Schoell M.; Sessions A.L.; Eiler J.M.
发表日期2014
ISSN0036-8075
起始页码1500
结束页码1503
卷号344期号:6191
英文摘要Methane is an important greenhouse gas and energy resource generated dominantly by methanogens at low temperatures and through the breakdown of organic molecules at high temperatures. However, methane-formation temperatures in nature are often poorly constrained. We measured formation temperatures of thermogenic and biogenic methane using a "clumped isotope" technique. Thermogenic gases yield formation temperatures between 157° and 221°C, within the nominal gas window, and biogenic gases yield formation temperatures consistent with their comparatively lower-temperature formational environments (<50°C). In systems where gases have migrated and other proxies for gas-generation temperature yield ambiguous results, methane clumped-isotope temperatures distinguish among and allow for independent tests of possible gas-formation models.
英文关键词isotope; methane; carbon; petroleum; biogenic emission; energy resource; greenhouse gas; isotopic analysis; methane; methanogenesis; temperature profile; article; biogenesis; energy resource; environmental factor; greenhouse gas; high temperature; low temperature; methanogen; priority journal; thermogenesis; bioremediation; biosynthesis; chemistry; Euryarchaeota; gas; heat; metabolism; microbiology; oil and gas field; temperature; theoretical model; Biodegradation, Environmental; Carbon Isotopes; Euryarchaeota; Gases; Hot Temperature; Methane; Models, Theoretical; Oil and Gas Fields; Petroleum; Temperature
语种英语
来源期刊Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/245631
作者单位Division of Geological and Planetary Sciences, California Institute of Technology, 1200 East California Boulevard, Pasadena, CA 91125, United States; ExxonMobil Upstream Research Company, Houston, TX, United States; Division of Geochemistry, Petrobras Research and Development Center (CENPES), Rio de Janeiro, RJ, Brazil; U.S. Geological Survey, Denver Federal Center, Denver, CO, United States; Department of Geology, Amherst College, Amherst, MA, United States; Power, Environmental, and Energy Research Institute, Covina, CA, United States; GasConsult International Inc, Berkeley, CA, United States
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Stolper D.A.,Lawson M.,Davis C.L.,et al. Formation temperatures of thermogenic and biogenic methane[J],2014,344(6191).
APA Stolper D.A..,Lawson M..,Davis C.L..,Ferreira A.A..,Santos Neto E.V..,...&Eiler J.M..(2014).Formation temperatures of thermogenic and biogenic methane.Science,344(6191).
MLA Stolper D.A.,et al."Formation temperatures of thermogenic and biogenic methane".Science 344.6191(2014).
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