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DOI10.1126/science.1191056
Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon
Pöschl U.; Martin S.T.; Sinha B.; Chen Q.; Gunthe S.S.; Huffman J.A.; Borrmann S.; Farmer D.K.; Garland R.M.; Helas G.; Jimenez J.L.; King S.M.; Manzi A.; Mikhailov E.; Pauliquevis T.; Petters M.D.; Prenni A.J.; Roldin P.; Rose D.; Schneider J.; Su H.; Zorn S.R.; Artaxo P.; Andreae M.O.
发表日期2010
ISSN0036-8075
起始页码1513
结束页码1516
卷号329期号:5998
英文摘要The Amazon is one of the few continental regions where atmospheric aerosol particles and their effects on climate are not dominated by anthropogenic sources. During the wet season, the ambient conditions approach those of the pristine pre-industrial era. We show that the fine submicrometer particles accounting for most cloud condensation nuclei are predominantly composed of secondary organic material formed by oxidation of gaseous biogenic precursors. Supermicrometer particles, which are relevant as ice nuclei, consist mostly of primary biological material directly released from rainforest biota. The Amazon Basin appears to be a biogeochemical reactor, in which the biosphere and atmospheric photochemistry produce nuclei for clouds and precipitation sustaining the hydrological cycle. The prevailing regime of aerosol-cloud interactions in this natural environment is distinctly different from polluted regions.
英文关键词ice; nucleic acid; organic compound; aerosol composition; atmosphere-biosphere interaction; atmospheric chemistry; biogenic material; cloud condensation nucleus; hydrological cycle; particle size; photochemistry; precipitation (climatology); rainforest; aerosol; air pollution; article; atmosphere; biogeochemical cycle; bioreactor; biosphere; biota; cloud; gas; hydrology; nonhuman; oxidation; particle size; photochemistry; polymerization; precipitation; priority journal; rain forest; Amazon Basin
语种英语
来源期刊Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/245121
作者单位Max Planck Institute for Chemistry, 55128 Mainz, Germany; School of Engineering and Applied Sciences, Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA 02138, United States; Department of Chemistry and Biochemistry, Cooperative Institute for Research in Environmental Science, University of Colorado, Boulder, CO 80309, United States; National Institute of Amazonian Research, 69060 Manaus, Brazil; Atmospheric Physics Department, Institute of Physics, St. Petersburg State University, 198904 St. Petersburg, Russian Federation; Institute of Physics, University of São Paulo, 05508 São Paulo, Brazil; Federal University of São Paulo, 04023 Diadema, Brazil; Department of Atmospheric Science, Colorado State University, Fort Collins, CO 80523, United States; Marine Earth and Atmospheric Science, North Carolina State University, Raleigh, NC 27695, United States; Department of Physics, Lund University, 22100 Lund, Sweden
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Pöschl U.,Martin S.T.,Sinha B.,et al. Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon[J],2010,329(5998).
APA Pöschl U..,Martin S.T..,Sinha B..,Chen Q..,Gunthe S.S..,...&Andreae M.O..(2010).Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon.Science,329(5998).
MLA Pöschl U.,et al."Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon".Science 329.5998(2010).
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