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DOI | 10.1126/science.1103491 |
Organic aerosol growth mechanisms and their climate-forcing implications | |
Maria S.F.; Russell L.M.; Gilles M.K.; Myneni S.C.B. | |
发表日期 | 2004 |
ISSN | 0036-8075 |
起始页码 | 1921 |
结束页码 | 1924 |
卷号 | 306期号:5703 |
英文摘要 | Surface- and volume-limited chemical reactions on and in atmospheric aerosol particles cause growth while changing organic composition by 13 to 24% per day. Many of these particles contain carbonaceous components from mineral dust and combustion emissions in Africa, Asia, and North America and reveal reaction rates that are three times slower than those typically used in climate models. These slower rates for converting from volatile or Hydrophobic to condensed and hygroscopic organic compounds increase carbonaceous particle burdens in climate models by 70%, producing organic aerosol climate forcings of as much as -0.8 watt per square meter cooling and +0.3 watt per square meter warming. |
英文关键词 | Chemical reactions; Climatology; Combustion; Cooling; Hydrophobicity; Organic compounds; Particulate emissions; Carbonaceous components; Growth mechanisms; Organic compositions; Aerosols; carbon; organic compound; aerosol; climate forcing; growth; organic compound; aerosol; article; atmosphere; chemical composition; chemical reaction; climate change; combustion; cooling; hydrophobicity; mineral dust; polymerization; priority journal; volatilization; warming; wettability |
语种 | 英语 |
来源期刊 | Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/244658 |
作者单位 | Department of Chemical Engineering, Princeton University, Princeton, NJ 08544, United States; Department of Geosciences, Princeton University, Princeton, NJ 08544, United States; Scripps Institution of Oceanography, University of California San Diego, San Diego, CA 92093, United States; Chemical Sciences Division, Lawrence Berkeley Natl. Laboratory, Berkeley, CA 94720, United States; Advanced Light Source, Lawrence Berkeley Natl. Laboratory, Berkeley, CA 94720, United States |
推荐引用方式 GB/T 7714 | Maria S.F.,Russell L.M.,Gilles M.K.,et al. Organic aerosol growth mechanisms and their climate-forcing implications[J],2004,306(5703). |
APA | Maria S.F.,Russell L.M.,Gilles M.K.,&Myneni S.C.B..(2004).Organic aerosol growth mechanisms and their climate-forcing implications.Science,306(5703). |
MLA | Maria S.F.,et al."Organic aerosol growth mechanisms and their climate-forcing implications".Science 306.5703(2004). |
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