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DOI10.1126/science.258.5079.117
Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2
Lelieveld J.; Heintzenberg J.
发表日期1992
ISSN0036-8075
起始页码117
结束页码120
卷号258期号:5079
英文摘要Anthropogenic SO2 emissions may exert a significant cooling effect on climate in the Northern Hemisphere through backscattering of solar radiation by sulfate particles. Earlier estimates of the sulfate climate forcing were based on a limited number of sulfate-scattering correlation measurements from which a high sulfate-scattering efficiency was derived. Model results suggest that cloud processing of air is the underlying mechanism. Aqueous phase oxidation of SO2 into sulfate and the subsequent release of the dry aerosol by cloud evaporation render sulfate a much more efficient scatterer than through gas-phase SO2 oxidation.
英文关键词sulfur dioxide; article; climate; priority journal; solar radiation; aerosol; anthropogenic; climate; cloud oxidation; cooling effect; sulphate; sulphur dioxide
语种英语
来源期刊Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/244493
作者单位Max-Planck Institute for Chemistry, Atmospheric Chemistry Division, Post Office Box 3060, D-6500 Mainz, Germany; Department of Meteorology, University of Stockholm, S-10691 Stockholm, Sweden
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Lelieveld J.,Heintzenberg J.. Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2[J],1992,258(5079).
APA Lelieveld J.,&Heintzenberg J..(1992).Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2.Science,258(5079).
MLA Lelieveld J.,et al."Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2".Science 258.5079(1992).
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