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DOI | 10.1126/science.258.5079.117 |
Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2 | |
Lelieveld J.; Heintzenberg J. | |
发表日期 | 1992 |
ISSN | 0036-8075 |
起始页码 | 117 |
结束页码 | 120 |
卷号 | 258期号:5079 |
英文摘要 | Anthropogenic SO2 emissions may exert a significant cooling effect on climate in the Northern Hemisphere through backscattering of solar radiation by sulfate particles. Earlier estimates of the sulfate climate forcing were based on a limited number of sulfate-scattering correlation measurements from which a high sulfate-scattering efficiency was derived. Model results suggest that cloud processing of air is the underlying mechanism. Aqueous phase oxidation of SO2 into sulfate and the subsequent release of the dry aerosol by cloud evaporation render sulfate a much more efficient scatterer than through gas-phase SO2 oxidation. |
英文关键词 | sulfur dioxide; article; climate; priority journal; solar radiation; aerosol; anthropogenic; climate; cloud oxidation; cooling effect; sulphate; sulphur dioxide |
语种 | 英语 |
来源期刊 | Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/244493 |
作者单位 | Max-Planck Institute for Chemistry, Atmospheric Chemistry Division, Post Office Box 3060, D-6500 Mainz, Germany; Department of Meteorology, University of Stockholm, S-10691 Stockholm, Sweden |
推荐引用方式 GB/T 7714 | Lelieveld J.,Heintzenberg J.. Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2[J],1992,258(5079). |
APA | Lelieveld J.,&Heintzenberg J..(1992).Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2.Science,258(5079). |
MLA | Lelieveld J.,et al."Sulfate cooling effect on climate through in-cloud oxidation of anthropogenic SO2".Science 258.5079(1992). |
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