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DOI | 10.1126/science.276.5318.1530 |
The source of green light emission determined from a heavy-ion storage ring experiment | |
Kella D.; Vejby-Christensen L.; Johnson P.J.; Pedersen H.B.; Andersen L.H. | |
发表日期 | 1997 |
ISSN | 0036-8075 |
起始页码 | 1530 |
结束页码 | 1533 |
卷号 | 276期号:5318 |
英文摘要 | The final electronic states of oxygen atoms formed by dissociative recombination of O2+ with cold electrons have been measured by an imaging technique at a heavy-ion storage ring. The 3P, 1D, and 1S quantum yield for O2+ in the vibrational ground level was found to be 0.86, 1.09, and 0.05, respectively. The yield of the 1S state, which is responsible for the 5577 angstrom green light from upper planetary atmospheres, was more than an order of magnitude larger than the theoretical value used in atmospheric models. The results may help refine the models of the chemistry and dynamics of the ionosphere and provide guidance for further quantum-chemistry calculations.The final electronic states of oxygen atoms formed by dissociative recombination of O2+ with cold electrons have been measured by an imaging technique at a heavy-ion storage ring. The 3P, 1D, and 1S quantum yield for O2+ in the vibrational ground level was found to be 0.86, 1.09, and 0.05, respectively. The yield of the 1S state, which is responsible for the 5577 angstrom green light from upper planetary atmospheres, was more than an order of magnitude larger than the theoretical value used in atmospheric models. The results may help refine the models of the chemistry and dynamics of the ionosphere and provide guidance for further quantum-chemistry calculations. |
英文关键词 | Atoms; Dissociation; Electron energy levels; Electrons; Imaging techniques; Ions; Molecules; Oxygen; Storage rings; Dissociative recombination; Green light emission; Quantum chemistry; Quantum yield; Ionosphere; article; atmosphere; dissociation; infrared radiation; ion transport; priority journal; quantum chemistry; ultraviolet radiation |
语种 | 英语 |
来源期刊 | Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/244248 |
作者单位 | Institute of Physics and Astronomy, University of Aarhus, DK 8000, Aarhus C, Denmark |
推荐引用方式 GB/T 7714 | Kella D.,Vejby-Christensen L.,Johnson P.J.,et al. The source of green light emission determined from a heavy-ion storage ring experiment[J],1997,276(5318). |
APA | Kella D.,Vejby-Christensen L.,Johnson P.J.,Pedersen H.B.,&Andersen L.H..(1997).The source of green light emission determined from a heavy-ion storage ring experiment.Science,276(5318). |
MLA | Kella D.,et al."The source of green light emission determined from a heavy-ion storage ring experiment".Science 276.5318(1997). |
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