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DOI10.1126/science.276.5318.1530
The source of green light emission determined from a heavy-ion storage ring experiment
Kella D.; Vejby-Christensen L.; Johnson P.J.; Pedersen H.B.; Andersen L.H.
发表日期1997
ISSN0036-8075
起始页码1530
结束页码1533
卷号276期号:5318
英文摘要The final electronic states of oxygen atoms formed by dissociative recombination of O2+ with cold electrons have been measured by an imaging technique at a heavy-ion storage ring. The 3P, 1D, and 1S quantum yield for O2+ in the vibrational ground level was found to be 0.86, 1.09, and 0.05, respectively. The yield of the 1S state, which is responsible for the 5577 angstrom green light from upper planetary atmospheres, was more than an order of magnitude larger than the theoretical value used in atmospheric models. The results may help refine the models of the chemistry and dynamics of the ionosphere and provide guidance for further quantum-chemistry calculations.The final electronic states of oxygen atoms formed by dissociative recombination of O2+ with cold electrons have been measured by an imaging technique at a heavy-ion storage ring. The 3P, 1D, and 1S quantum yield for O2+ in the vibrational ground level was found to be 0.86, 1.09, and 0.05, respectively. The yield of the 1S state, which is responsible for the 5577 angstrom green light from upper planetary atmospheres, was more than an order of magnitude larger than the theoretical value used in atmospheric models. The results may help refine the models of the chemistry and dynamics of the ionosphere and provide guidance for further quantum-chemistry calculations.
英文关键词Atoms; Dissociation; Electron energy levels; Electrons; Imaging techniques; Ions; Molecules; Oxygen; Storage rings; Dissociative recombination; Green light emission; Quantum chemistry; Quantum yield; Ionosphere; article; atmosphere; dissociation; infrared radiation; ion transport; priority journal; quantum chemistry; ultraviolet radiation
语种英语
来源期刊Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/244248
作者单位Institute of Physics and Astronomy, University of Aarhus, DK 8000, Aarhus C, Denmark
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Kella D.,Vejby-Christensen L.,Johnson P.J.,et al. The source of green light emission determined from a heavy-ion storage ring experiment[J],1997,276(5318).
APA Kella D.,Vejby-Christensen L.,Johnson P.J.,Pedersen H.B.,&Andersen L.H..(1997).The source of green light emission determined from a heavy-ion storage ring experiment.Science,276(5318).
MLA Kella D.,et al."The source of green light emission determined from a heavy-ion storage ring experiment".Science 276.5318(1997).
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