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DOI10.1126/science.1164015
Photosynthetic control of atmospheric carbonyl sulfide during the growing season
Campbell J.E.; Carmichael G.R.; Chai T.; Mena-Carrasco M.; Tang Y.; Blake D.R.; Blake N.J.; Vay S.A.; Collatz G.J.; Baker I.; Berry J.A.; Montzka S.A.; Sweeney C.; Schnoor J.L.; Stanier C.O.
发表日期2008
ISSN0036-8075
起始页码1085
结束页码1088
卷号322期号:5904
英文摘要Climate models incorporate photosynthesis-climate feedbacks, yet we lack robust tools for large-scale assessments of these processes. Recent work suggests that carbonyl sulfide (COS), a trace gas consumed by plants, could provide a valuable constraint on photosynthesis. Here we analyze airborne observations of COS and carbon dioxide concentrations during the growing season over North America with a three-dimensional atmospheric transport model. We successfully modeled the persistent vertical drawdown of atmospheric COS using the quantitative relation between COS and photosynthesis that has been measured in plant chamber experiments. Furthermore, this drawdown is driven by plant uptake rather than other continental and oceanic fluxes in the model. These results provide quantitative evidence that COS gradients in the continental growing season may have broad use as a measurement-based photosynthesis tracer.
英文关键词carbon dioxide; carbonyl derivative; sulfide; atmospheric transport; carbon dioxide; carbonyl compound; climate modeling; concentration (composition); growing season; photosynthesis; article; atmospheric transport; chemical analysis; concentration (parameters); ecosystem; growing season; outcome assessment; photosynthesis; priority journal; Atmosphere; Carbon Dioxide; North America; Photosynthesis; Plants; Seasons; Sulfur Oxides
语种英语
来源期刊Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/243221
作者单位Department of Civil and Environmental Engineering, University of Iowa, Iowa City, IA 52242, United States; Center for Global and Regional Environmental Research, University of Iowa, Iowa City, IA 52242, United States; Science and Technology Corporation, Hampton, VA 23666, United States; Department of Environmental Engineering, Universidad Andrés Bello, Santiago, Chile; Molina Center for Energy and the Environment, Massachusetts Institute of Technology, Cambridge, MA 02139, United States; Department of Chemistry, University of California, Irvine, CA 92697, United States; NASA Langley Research Center, Hampton, VA 23681, United States; Biospheric Sciences Branch, NASA-Goddard Space Flight Center, Greenbelt, MD 20771, United States; Department of Atmospheric Science, Colorado State University, Fort Collins, CO 80523, United States; Department of Global Ecology, Carnegie Institution of Washington, Stanford, CA 94305, United States; Global Monitoring Division, National Oceanic and Atmospheric Administration (NO...
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Campbell J.E.,Carmichael G.R.,Chai T.,et al. Photosynthetic control of atmospheric carbonyl sulfide during the growing season[J],2008,322(5904).
APA Campbell J.E..,Carmichael G.R..,Chai T..,Mena-Carrasco M..,Tang Y..,...&Stanier C.O..(2008).Photosynthetic control of atmospheric carbonyl sulfide during the growing season.Science,322(5904).
MLA Campbell J.E.,et al."Photosynthetic control of atmospheric carbonyl sulfide during the growing season".Science 322.5904(2008).
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