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DOI10.1016/j.scib.2019.11.021
Enhancement of superconductivity in organic-inorganic hybrid topological materials
Zhang H.; Rousuli A.; Shen S.; Zhang K.; Wang C.; Luo L.; Wang J.; Wu Y.; Xu Y.; Duan W.; Yao H.; Yu P.; Zhou S.
发表日期2020
ISSN20959273
起始页码188
结束页码193
卷号65期号:3
英文摘要Inducing or enhancing superconductivity in topological materials is an important route toward topological superconductivity. Reducing the thickness of transition metal dichalcogenides (e.g. WTe2 and MoTe2) has provided an important pathway to engineer superconductivity in topological matters. However, such monolayer sample is difficult to obtain, unstable in air, and with extremely low Tc. Here we report an experimentally convenient approach to control the interlayer coupling to achieve tailored topological properties, enhanced superconductivity and good sample stability through organic-cation intercalation of the Weyl semimetals MoTe2 and WTe2. The as-formed organic-inorganic hybrid crystals are weak topological insulators with enhanced Tc of 7.0 K for intercalated MoTe2 (0.25 K for pristine crystal) and 2.3 K for intercalated WTe2 (2.8 times compared to monolayer WTe2). Such organic-cation intercalation method can be readily applied to many other layered crystals, providing a new pathway for manipulating their electronic, topological and superconducting properties. © 2019 Science China Press
关键词Enhanced superconductivityIntercalation of organic cationIonic liquids cationsOrganic-inorganic hybrid materialsTopological materialsWeyl semimetals MoTe2 and WTe2
英文关键词Ionic liquids; Molybdenum compounds; Monolayers; organic-inorganic materials; Positive ions; Tellurium compounds; Topology; Transition metals; Organic cations; Organic-inorganic hybrid; Organic-inorganic hybrid crystals; Organic-inorganic hybrid materials; Superconducting properties; Topological materials; Transition metal dichalcogenides; Weyl semimetals MoTe2 and WTe2; Tungsten compounds
语种英语
来源期刊Science Bulletin
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/207294
作者单位State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, 100084, China; Department of Mechanical Engineering and Tsinghua-Foxconn Nanotechnology Research Center, Tsinghua University, Beijing, 100084, China; Frontier Science Center for Quantum Information, Beijing, 100084, China; Institute for Advanced Study, Tsinghua University, Beijing, 100084, China
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GB/T 7714
Zhang H.,Rousuli A.,Shen S.,et al. Enhancement of superconductivity in organic-inorganic hybrid topological materials[J],2020,65(3).
APA Zhang H..,Rousuli A..,Shen S..,Zhang K..,Wang C..,...&Zhou S..(2020).Enhancement of superconductivity in organic-inorganic hybrid topological materials.Science Bulletin,65(3).
MLA Zhang H.,et al."Enhancement of superconductivity in organic-inorganic hybrid topological materials".Science Bulletin 65.3(2020).
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