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DOI10.1039/d0ee02981e
Recent advances in innovative strategies for the CO2electroreduction reaction
Tan X.; Yu C.; Ren Y.; Cui S.; Li W.; Qiu J.
发表日期2021
ISSN17545692
起始页码765
结束页码780
卷号14期号:2
英文摘要The carbon dioxide electroreduction reaction (CO2RR), an emerging electrocatalysis reaction, is promising for converting CO2 into value-added fuels or chemicals (e.g., hydrocarbons and oxygenates). However, the CO2RR system for practical evaluations and applications is still limited by its low current density and poor CO2 utilization and conversion as well as dismal energy efficiency. To reach up to the practical application level, the components of the CO2RR device/system need to be systematically considered and optimized. This review specifically focuses on the latest and innovative design strategies toward each part of the system. In particular, the innovative and idiographic design strategies for tandem catalysts, promising electrolytes, upgraded electrodes, and advanced devices as well as anodic reactions are discussed at length. Moreover, some individual perspectives on opportunities and future challenges for each component of the CO2RR system are also provided. Perspectives and new trends presented in this review are not just labels and classifications. Instead, it is particularly expected that innovative ideas and visionary discussions in this review can systematically instruct and inspire researchers to contribute more efforts toward comprehensively optimizing the performance of the CO2RR system to a higher level. © The Royal Society of Chemistry.
英文关键词Conversion efficiency; Electrocatalysis; Electrolytic reduction; Energy efficiency; Application level; Design strategies; Electro reduction; Future challenges; Innovative design; Innovative ideas; Innovative strategies; Low current density; Carbon dioxide; carbon dioxide; electrochemical method; electrode; electronic equipment; energy efficiency; equipment; performance assessment; reduction
语种英语
来源期刊Energy & Environmental Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/190791
作者单位State Key Lab of Fine Chemicals, School of Chemical Engineering, Liaoning Key Lab for Energy Materials and Chemical Engineering, Dalian University of Technology, Dalian, 116024, China; College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
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GB/T 7714
Tan X.,Yu C.,Ren Y.,et al. Recent advances in innovative strategies for the CO2electroreduction reaction[J],2021,14(2).
APA Tan X.,Yu C.,Ren Y.,Cui S.,Li W.,&Qiu J..(2021).Recent advances in innovative strategies for the CO2electroreduction reaction.Energy & Environmental Science,14(2).
MLA Tan X.,et al."Recent advances in innovative strategies for the CO2electroreduction reaction".Energy & Environmental Science 14.2(2021).
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