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DOI | 10.1039/d0ee03300f |
Solar fuels and feedstocks: The quest for renewable black gold | |
Sayre H.J.; Tian L.; Son M.; Hart S.M.; Liu X.; Arias-Rotondo D.M.; Rand B.P.; Schlau-Cohen G.S.; Scholes G.D. | |
发表日期 | 2021 |
ISSN | 17545692 |
起始页码 | 1402 |
结束页码 | 1419 |
卷号 | 14期号:3 |
英文摘要 | Photocatalysis for organic synthesis is a tool capable of C-C, C-O and C-N bond transformations. This technology has the potential to transform the chemical manufacturing industry and support growing demand for chemical feedstocks. Compared to traditional catalysis, photocatalysis can access alternative reaction pathways that lower the overall energy requirement and operate at or near ambient conditions. A key challenge is the delivery of photoenergy at the scale required for rapid and efficient operation of the catalyst. The development of efficient, broad-spectrum light harvesting devices that funnel light energy to a catalyst, along with catalyst design to selectively enable high-energy reactions, are necessary steps towards solar fuels and feedstocks. This perspective highlights some recent advances in photocatalysis and advocates for expanding the scope of photocatalysis for large-scale industrial applications. © 2021 The Royal Society of Chemistry. |
英文关键词 | Catalysts; Feedstocks; Gold; Light; Ambient conditions; Catalyst designs; Chemical feedstocks; Chemical manufacturing industries; Energy requirements; Light-harvesting; Organic synthesis; Reaction pathways; Photocatalysis; fuel; gold; renewable resource; solar power |
语种 | 英语 |
来源期刊 | Energy & Environmental Science
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文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/190737 |
作者单位 | Department of Chemistry, Princeton University, Princeton, NJ, United States; Department of Chemistry, University of Wisconsin-Madison, Madison, WI, United States; Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA, United States; Department of Electrical Engineering, Princeton University, Princeton, NJ, United States; Department of Chemistry, Kalamazoo College, Kalamazoo, MI, United States |
推荐引用方式 GB/T 7714 | Sayre H.J.,Tian L.,Son M.,et al. Solar fuels and feedstocks: The quest for renewable black gold[J],2021,14(3). |
APA | Sayre H.J..,Tian L..,Son M..,Hart S.M..,Liu X..,...&Scholes G.D..(2021).Solar fuels and feedstocks: The quest for renewable black gold.Energy & Environmental Science,14(3). |
MLA | Sayre H.J.,et al."Solar fuels and feedstocks: The quest for renewable black gold".Energy & Environmental Science 14.3(2021). |
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