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DOI	10.1039/d1ee00142f
	Pyrolyzed M-N: Xcatalysts for oxygen reduction reaction: Progress and prospects
	Luo E.; Chu Y.; Liu J.; Shi Z.; Zhu S.; Gong L.; Ge J.; Choi C.H.; Liu C.; Xing W.
发表日期	2021
ISSN	17545692
起始页码	2158
结束页码	2185
卷号	14 期号:4
英文摘要	Fuel cells, a sustainable technology that assures a cleaner earth, once experienced disillusion due to the issue of economic viability associated with the massive usage of Pt-based catalysts. To address this issue, research on cost-effective catalysts, especially on the cathode side, has been intensively carried out where the latest achievements have made the M-Nx/C material on its verge of application. Here, we present a comprehensive overview of the fundamental chemistry of oxygen reduction reaction (ORR) and the progress of the M-Nx/C catalysts. Efforts aimed at clarifying the nature of catalytic sites are summarized, highlighting the indispensable role of advanced characterization tools. A variety of successful attempts are exemplified to describe the synthetic methodologies, followed by close tracking of newly emerging single-atom or dual-atom sites. Future directions for this research area are believed to be the rational and/or controllable synthesis of catalysts with adequate active sites and the use of strategies to substantially alleviate catalyst degradation. This journal is © The Royal Society of Chemistry.
英文关键词	Cost effectiveness; Electrolytic reduction; Fuel cells; Oxygen; Oxygen reduction reaction; Catalyst degradation; Catalytic sites; Characterization tools; Controllable synthesis; Economic viability; Pt-based catalyst; Sustainable technology; Synthetic methodology; Catalyst activity; electrochemical method; electrode; energy storage
语种	英语
来源期刊	Energy & Environmental Science
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/190708
作者单位	State Key Laboratory of Electroanalytical Chemistry, Jilin Province Key Laboratory of Low Carbon Chemical Power, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun Jilin, 130022, China; School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei Anhui, 230026, China; School of Materials Science and Engineering, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea
推荐引用方式 GB/T 7714	Luo E.,Chu Y.,Liu J.,et al. Pyrolyzed M-N: Xcatalysts for oxygen reduction reaction: Progress and prospects[J],2021,14(4).
APA	Luo E..,Chu Y..,Liu J..,Shi Z..,Zhu S..,...&Xing W..(2021).Pyrolyzed M-N: Xcatalysts for oxygen reduction reaction: Progress and prospects.Energy & Environmental Science,14(4).
MLA	Luo E.,et al."Pyrolyzed M-N: Xcatalysts for oxygen reduction reaction: Progress and prospects".Energy & Environmental Science 14.4(2021).