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DOI10.1039/c7ee00601b
Interface design for high-efficiency non-fullerene polymer solar cells
Sun C.; Wu Z.; Hu Z.; Xiao J.; Zhao W.; Li H.-W.; Li Q.-Y.; Tsang S.-W.; Xu Y.-X.; Zhang K.; Yip H.-L.; Hou J.; Huang F.; Cao Y.
发表日期2017
ISSN17545692
起始页码1784
结束页码1791
卷号10期号:8
英文摘要Non-fullerene polymer solar cells have attracted extensive attention due to their potential for overcoming the performance bottleneck currently encountered in fullerene-based photovoltaics. Herein, we report non-fullerene polymer solar cells with a maximal power conversion efficiency of over 11% by introducing an n-type water/alcohol soluble conjugated polymer as a cathode interlayer. We found that the contact between the n-type interlayer and the donor provides an extra interface for charge dissociation and the matching of energy levels between the n-type interlayer and the acceptor allows efficient electron extraction from the bulk heterojunction, which eventually leads to much improved performance. This study proposes a significant design rule for designing new interfaces for high performance non-fullerene photovoltaics. © The Royal Society of Chemistry 2017.
英文关键词Conjugated polymers; Fullerenes; Heterojunctions; Polymer solar cells; Software design; Solar power generation; Bulk heterojunction; Cathode interlayers; Electron extraction; High-efficiency; Interface designs; Performance bottlenecks; Photovoltaics; Power conversion efficiencies; Solar cells
语种英语
来源期刊Energy & Environmental Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/190445
作者单位Institute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou, 510640, China; State Key Laboratory of Polymer Physics and Chemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China; Department of Physics and Materials Science, City University of Hong Kong, Kowloon Tong, Hong Kong; College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu, 610065, China
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GB/T 7714
Sun C.,Wu Z.,Hu Z.,et al. Interface design for high-efficiency non-fullerene polymer solar cells[J],2017,10(8).
APA Sun C..,Wu Z..,Hu Z..,Xiao J..,Zhao W..,...&Cao Y..(2017).Interface design for high-efficiency non-fullerene polymer solar cells.Energy & Environmental Science,10(8).
MLA Sun C.,et al."Interface design for high-efficiency non-fullerene polymer solar cells".Energy & Environmental Science 10.8(2017).
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