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DOI10.1039/c8ee00162f
Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells
Lee J.-H.; Kim J.; Kim G.; Shin D.; Jeong S.Y.; Lee J.; Hong S.; Choi J.W.; Lee C.-L.; Kim H.; Yi Y.; Lee K.
发表日期2018
ISSN17545692
起始页码1742
结束页码1751
卷号11期号:7
英文摘要Elimination of charge trapping at defects is highly challenging for poly-crystalline organometal halide perovskites. Here, we report a new architecture for reinforcing the built-in electric field (Ein) across the photoactive layer with a pair of strong electric dipole layers (EDLs). The paired EDLs significantly intensify the Ein across the perovskite layer, resulting in suppressed charge trapping of photogenerated charges. As a result, our low-temperature processed P-I-N planar PeSC devices using the paired EDLs exhibit a higher power conversion efficiency (ηmax ∼ 19.4%) and a smaller device-to-device variation with a standard deviation (S.D.) of 0.70%, which far surpass those (ηmax ∼ 17.8%, S.D. ∼ 1.1%) of the devices with typical charge transport layers. © 2018 The Royal Society of Chemistry.
英文关键词Charge trapping; Electric fields; Heterojunction bipolar transistors; Perovskite; Solar cells; Temperature; Built-in electric fields; Charge transport layer; Electric dipole layer; Halide perovskites; Photoactive layers; Photogenerated charge; Power conversion efficiencies; Standard deviation; Perovskite solar cells; efficiency measurement; electric field; equipment; fuel cell; low temperature; perovskite; polymer; temperature effect
语种英语
来源期刊Energy & Environmental Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/190202
作者单位School of Materials Science and Engineering, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Heeger Center for Advanced Materials, Research Institute for Solar and Sustainable Energies, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Institute of Physics and Applied Physics, Van der Waals Materials Research Center, Yonsei University, Seoul, 03722, South Korea; Advanced Photonics Research Institute, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Institute of Integrated Technology, Gwangju Institute of Science and Technology, Gwangju, 61005, South Korea; Department of Electrical and Computer Engineering, University of Toronto, 10 King's College Road, Toronto, ON M5S 3G4, Canada
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Lee J.-H.,Kim J.,Kim G.,et al. Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells[J],2018,11(7).
APA Lee J.-H..,Kim J..,Kim G..,Shin D..,Jeong S.Y..,...&Lee K..(2018).Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells.Energy & Environmental Science,11(7).
MLA Lee J.-H.,et al."Introducing paired electric dipole layers for efficient and reproducible perovskite solar cells".Energy & Environmental Science 11.7(2018).
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