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DOI | 10.1039/c8ee01564c |
Ternary non-fullerene polymer solar cells with 13.51% efficiency and a record-high fill factor of 78.13% | |
Nian L.; Kan Y.; Wang H.; Gao K.; Xu B.; Rong Q.; Wang R.; Wang J.; Liu F.; Chen J.; Zhou G.; Russell T.P.; Jen A.K.-Y. | |
发表日期 | 2018 |
ISSN | 17545692 |
起始页码 | 3392 |
结束页码 | 3399 |
卷号 | 11期号:12 |
英文摘要 | Non-fullerene polymer solar cells (NF PSCs) have attracted much attention in recent years due to their rapidly increasing power conversion efficiency (PCE). In this work, two highly efficient ternary NF PSCs with FFs over 78% and PCEs up to 13.52% and 12.70% are demonstrated by adding a strongly aggregating polymer P1 into the classic PBDB-T:IT-M and PBDB-T:ITIC non-fullerene blends. The addition of P1 significantly enhances the crystallization of the blend film, while maintaining the desired morphology. The ternary devices show highly improved charge extraction and suppressed charge recombination in comparison to the binary mixture. The PCE of the PBDB-T:ITIC based NF PSC was found to increase from 10.82% to 12.70% and the FF from 71.85% to 78.07% after adding P1. For the PBDB-T:IT-M based NF PSC, the PCE increases from 11.71% to 13.52% and the FF from 72.07% to 77.83%. The high FFs and PCEs are the best results reported for ternary NF PSCs to date. © 2018 The Royal Society of Chemistry. |
英文关键词 | Binary mixtures; Efficiency; Fullerenes; Polymer blends; Solar cells; Blend films; Charge extraction; Charge recombinations; High fill factors; Power conversion efficiencies; Polymer solar cells; crystallization; energy efficiency; extraction method; film; fuel cell; polymer; recombination; Anatomy; Conversion; Crystallization; Efficiency; Film; Mixtures; Records; Solar Cells |
语种 | 英语 |
来源期刊 | Energy & Environmental Science |
文献类型 | 期刊论文 |
条目标识符 | http://gcip.llas.ac.cn/handle/2XKMVOVA/190049 |
作者单位 | Guangdong Provincial Key Laboratory of Optical Information Materials and Technology, Institute of Electronic Paper Displays, South China Academy of Advanced Optoelectronics, South China Normal University, Guangzhou, 510006, China; National Center for International Research on Green Optoelectronics, South China Normal University, Guangzhou, 510006, China; Department of Materials Science and Engineering, University of Washington, Seattle, WA 98195, United States; Institute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou, 510640, China; Department of Physics and Astronomy, Collaborative Innovation Center of IFSA (CICIFSA), Shanghai Jiaotong University, Shanghai, 200240, China; Materials Sciences Division, Lawrence Berkeley National Lab, Berkeley, CA 94720, United States; Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong |
推荐引用方式 GB/T 7714 | Nian L.,Kan Y.,Wang H.,et al. Ternary non-fullerene polymer solar cells with 13.51% efficiency and a record-high fill factor of 78.13%[J],2018,11(12). |
APA | Nian L..,Kan Y..,Wang H..,Gao K..,Xu B..,...&Jen A.K.-Y..(2018).Ternary non-fullerene polymer solar cells with 13.51% efficiency and a record-high fill factor of 78.13%.Energy & Environmental Science,11(12). |
MLA | Nian L.,et al."Ternary non-fullerene polymer solar cells with 13.51% efficiency and a record-high fill factor of 78.13%".Energy & Environmental Science 11.12(2018). |
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