气候变化领域集成服务门户(CCPortal): Principles of photothermal gas-phase heterogeneous CO2 catalysis

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DOI	10.1039/c8ee02790k
	Principles of photothermal gas-phase heterogeneous CO2 catalysis
	Ghoussoub M.; Xia M.; Duchesne P.N.; Segal D.; Ozin G.
发表日期	2019
ISSN	17545692
起始页码	1122
结束页码	1142
卷号	12 期号:4
英文摘要	Photothermal catalysis is an emerging sub-discipline of heterogeneous catalysis. It is distinct from both thermochemical catalysis driven by heat and photochemical catalysis powered by sunlight. Instead, photothermal catalysis exploits broad absorption of the solar spectrum to stimulate a combination of thermochemical and photochemical processes, which contribute synergistically to driving catalytic reactions. In particular, it is proving an effective and promising strategy for converting CO2 to synthetic fuels. This article provides a critical appraisal of the concepts and principles underpinning the theory and practice of photothermal CO2 catalysis. Ultimately, the goal is to gain an appreciation of the scientific, technological, economic, and environmental challenges inevitably confronted by those pursuing the development of photothermal CO2 refineries. © 2019 The Royal Society of Chemistry.
英文关键词	Absorption spectroscopy; Carbon dioxide; Photochemical reactions; Synthetic fuels; Broad absorptions; Catalytic reactions; Environmental challenges; Photochemical catalysis; Photochemical process; Solar spectrum; Sub-disciplines; Theory and practice; Catalysis; absorption; carbon dioxide; catalysis; gas exchange; photochemistry; synergism; thermochemistry
语种	英语
来源期刊	Energy & Environmental Science
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/189951
作者单位	GAO Materials Chemistry Group, Department of Chemistry, University of Toronto, 80 St George Street, Toronto, ON M5S 3H6, Canada; Chemical Physics Theory Group, Department of Chemistry, University of Toronto, 80 St George Street, Toronto, ON M5S 3H6, Canada
推荐引用方式 GB/T 7714	Ghoussoub M.,Xia M.,Duchesne P.N.,et al. Principles of photothermal gas-phase heterogeneous CO2 catalysis[J],2019,12(4).
APA	Ghoussoub M.,Xia M.,Duchesne P.N.,Segal D.,&Ozin G..(2019).Principles of photothermal gas-phase heterogeneous CO2 catalysis.Energy & Environmental Science,12(4).
MLA	Ghoussoub M.,et al."Principles of photothermal gas-phase heterogeneous CO2 catalysis".Energy & Environmental Science 12.4(2019).