气候变化领域集成服务门户(CCPortal): Graphdiyne for crucial gas involved catalytic reactions in energy conversion applications

CCPortal

DOI	10.1039/c9ee03558c
	Graphdiyne for crucial gas involved catalytic reactions in energy conversion applications
	Li J.; Gao X.; Zhu L.; Ghazzal M.N.; Zhang J.; Tung C.-H.; Wu L.-Z.
发表日期	2020
ISSN	17545692
起始页码	1326
结束页码	1346
卷号	13 期号:5
英文摘要	Gas involved reactions including the oxygen evolution reaction (OER), hydrogen evolution reaction (HER), oxygen reduction reaction (ORR), nitrogen reduction reaction (NRR) and carbon dioxide reduction reaction (CO2RR) are the center of sustainable energy conversion technologies. Development of efficient catalysts to boost the aforementioned reactions is highly imperative because of the sluggish kinetics and large overpotential. Carbon-based catalysts have triggered huge interest in gas involved catalytic reactions owing to the low cost, high energy conversion efficiency and environmental friendliness. Graphdiyne (GDY), a rising-star carbon allotrope, consists of a highly π-conjugated structure of sp2- and sp-hybridized carbons. The unique electronic and topological structures and preparation advantages endow GDY with the possibilities to construct new-concept carbon-based catalysts for achieving high efficiency for energy conversion. Herein, a concise but comprehensive review of recent advances in the synthesis and applications of GDY based catalysts for crucial gas involved reactions is presented. Some new perspectives of opportunities and challenges in developing GDY-based catalysts for gas-involved energy conversion are also discussed. © The Royal Society 2020 of Chemistry.
英文关键词	Carbon dioxide; Catalysis; Catalysts; Electrolytic reduction; Gases; Organic polymers; Oxygen; Oxygen reduction reaction; Pollution control; Carbon based catalysts; Carbon dioxide reduction; Conjugated structures; Efficient catalysts; Environmental friendliness; High energy conversions; Oxygen evolution reaction (oer); Topological structure; Conversion efficiency; catalysis; catalyst; chemical compound; chemical reaction; energy budget
语种	英语
来源期刊	Energy & Environmental Science
文献类型	期刊论文
条目标识符	http://gcip.llas.ac.cn/handle/2XKMVOVA/189717
作者单位	Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing, 100190, China; University of Chinese Academy of Sciences, Beijing, 100190, China; Université Paris-Saclay, Cnrs, Laboratoire de Chimie Physique, Orsay, 91405, France; Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China
推荐引用方式 GB/T 7714	Li J.,Gao X.,Zhu L.,et al. Graphdiyne for crucial gas involved catalytic reactions in energy conversion applications[J],2020,13(5).
APA	Li J..,Gao X..,Zhu L..,Ghazzal M.N..,Zhang J..,...&Wu L.-Z..(2020).Graphdiyne for crucial gas involved catalytic reactions in energy conversion applications.Energy & Environmental Science,13(5).
MLA	Li J.,et al."Graphdiyne for crucial gas involved catalytic reactions in energy conversion applications".Energy & Environmental Science 13.5(2020).