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DOI10.1029/2019JD031837
Coral Reef Emissions of Atmospheric Dimethylsulfide and the Influence on Marine Aerosols in the Southern Great Barrier Reef, Australia
Jackson R.L.; Gabric A.J.; Woodhouse M.T.; Swan H.B.; Jones G.B.; Cropp R.; Deschaseaux E.S.M.
发表日期2020
ISSN2169897X
卷号125期号:7
英文摘要Variability in atmospheric dimethylsulfide (DMSa) and the potential influence on atmospheric aerosols was investigated at Heron Island in the southern Great Barrier Reef (GBR), Australia. This work compiles previously published DMSa data (reported in Swan, Jones, Deschaseaux, & Eyre, 2017, https://doi.org/10.1007/s00216-017-0385-8), with additional surveys of DMSa, atmospheric particle number concentration, and other oceanic and atmospheric data sets. DMSa was higher in summer (mean 3.2 nmol m−3/78 ppt) than winter (mean 1.3 nmol m−3/32 ppt), reflective of seasonal shifts in phytoplankton biomass and emissions from corals in the southern GBR. Seasonally extreme spikes in DMSa were detected during low tide and low wind speed, supporting findings that the coral reef can be an important source of DMSa above background oceanic emissions. A significant link was present between DMSa and aerosol concentration (ranging from 0.5 to 2.5 μm) during calm, daylight hours, when conditions were optimal for the local oxidation of DMSa to sulfate aerosol precursors. This link may reflect condensational growth of existing fine particles (< 0.5 μm), which is the dominant pathway by which biogenic trace gases influence aerosols in the marine boundary layer. Aerosol concentration significantly correlated with reduced surface solar irradiance and sea surface temperature, which is potential evidence of a local negative feedback mitigating coral physiological stress. These findings provide a step toward a better understanding of the processes influencing DMSa and aerosol concentrations and of the consequences for the local radiative balance over coral reefs; an increasingly important topic with ongoing ocean warming and coral bleaching. ©2020. The Authors.
英文关键词coral reef; dimethylsulfide; feedback; marine aerosols; thermal stress
语种英语
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/186062
作者单位School of Environment and Science, Griffith University, Gold Coast, QLD, Australia; Australian Rivers Institute, Griffith University, Gold Coast, QLD, Australia; School of Environment and Science, Griffith University, Nathan, QLD, Australia; Climate Science Centre, Oceans and Atmosphere, Commonwealth Scientific and Industrial Research Organisation, Aspendale, VIC, Australia; Centre for Coastal Biogeochemistry, School of Environment, Science and Engineering, Southern Cross University, Lismore, NSW, Australia
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Jackson R.L.,Gabric A.J.,Woodhouse M.T.,et al. Coral Reef Emissions of Atmospheric Dimethylsulfide and the Influence on Marine Aerosols in the Southern Great Barrier Reef, Australia[J],2020,125(7).
APA Jackson R.L..,Gabric A.J..,Woodhouse M.T..,Swan H.B..,Jones G.B..,...&Deschaseaux E.S.M..(2020).Coral Reef Emissions of Atmospheric Dimethylsulfide and the Influence on Marine Aerosols in the Southern Great Barrier Reef, Australia.Journal of Geophysical Research: Atmospheres,125(7).
MLA Jackson R.L.,et al."Coral Reef Emissions of Atmospheric Dimethylsulfide and the Influence on Marine Aerosols in the Southern Great Barrier Reef, Australia".Journal of Geophysical Research: Atmospheres 125.7(2020).
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