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DOI10.1029/2020JD033984
Trace Elements From Ocean-Going Vessels in East Asia: Vanadium and Nickel Emissions and Their Impacts on Air Quality
Zhao J.; Zhang Y.; Xu H.; Tao S.; Wang R.; Yu Q.; Chen Y.; Zou Z.; Ma W.
发表日期2021
ISSN2169897X
卷号126期号:8
英文摘要Vanadium (V) and nickel (Ni) are considered the most abundant trace metals in ship exhaust burning heavy fuel oils. This study is the first attempt to estimate the impact of V and Ni from shipping on air quality in East Asia for the year 2015. In this study, emission inventories of V and Ni from shipping and land-based sources were constructed and implemented into the revised aerosol module to simulate ambient V and Ni concentrations. Our results showed that ship emissions contributed the majority of vanadium and were important to nickel emissions in most coastal regions in East Asia, with the contributions exceeding 60% and approximately 40% in some regions, respectively. The simulated ambient V and Ni concentrations has been validated by the measurements, and the comparison revealed there was an obvious improvement (reducing the mean bias by 32%–63%) in the model performance of the V and Ni predictions after including shipping emissions. Our study filled the gaps of trace element contributions in coastal regions and implied that the impact of metals from shipping traffic on regional air quality is worthy of attention in East Asia. Although the International Maritime Organization (IMO) low-sulfur fuel policy has been implemented since 2020, the impact of shipping traffic on trace metals with respect to regional air quality is still important given heavy fuel oils being in use. © 2021. The Authors.
语种英语
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/185318
作者单位Department of Environmental Science and Engineering, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Fudan University, Shanghai, China; Zhuhai Fudan Innovation Institute, Zhuhai, China; Big Data Institute for Carbon Emission and Environmental Pollution, Fudan University, Shanghai, China; Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
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Zhao J.,Zhang Y.,Xu H.,et al. Trace Elements From Ocean-Going Vessels in East Asia: Vanadium and Nickel Emissions and Their Impacts on Air Quality[J],2021,126(8).
APA Zhao J..,Zhang Y..,Xu H..,Tao S..,Wang R..,...&Ma W..(2021).Trace Elements From Ocean-Going Vessels in East Asia: Vanadium and Nickel Emissions and Their Impacts on Air Quality.Journal of Geophysical Research: Atmospheres,126(8).
MLA Zhao J.,et al."Trace Elements From Ocean-Going Vessels in East Asia: Vanadium and Nickel Emissions and Their Impacts on Air Quality".Journal of Geophysical Research: Atmospheres 126.8(2021).
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