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DOI10.1029/2020JD033829
How Does a Pinatubo-Size Volcanic Cloud Reach the Middle Stratosphere?
Stenchikov G.; Ukhov A.; Osipov S.; Ahmadov R.; Grell G.; Cady-Pereira K.; Mlawer E.; Iacono M.
发表日期2021
ISSN2169897X
卷号126期号:10
英文摘要Volcanic explosions are the most critical replenishing mechanism of the stratospheric aerosol Junge layer. A fresh volcanic cloud comprises mostly sulfur-bearing gases, volcanic ash, and water vapor. It is commonly assumed that only sulfate aerosols remain in an aged volcanic cloud. Accurate simulation of the initial evolution of multicomponent fresh volcanic clouds is largely missing due to insufficient spatial resolution and a lack of relevant physics in global climate models. However, this initial stage is essential, as the vertical structure, composition, and altitude of a freshly developed volcanic cloud affect its long-term evolution. To fill this gap, we modified a regional WRF-Chem model to study the dispersion of a Pinatubo-size volcanic cloud in the equatorial belt with a 25 km grid spacing explicitly accounting for the SO2, ash, sulfate, water vapor, and hydrometeors radiative effects. The model best reproduces the observed evolution of the Pinatubo optical depth when eruptive products are injected above the cold tropical tropopause at 17 km. During the first week, the volcanic cloud in our simulations rises 1 km/day. Ash is primarily responsible for the heating and lofting of the volcanic products. Radiative heating of SO2 is weaker than that of ash and sulfate but is sufficient to position the core of the SO2 layer 1–2 km above the sulfate layer. Utilizing a more realistic description of the volcanic cloud's initial stage potentially improves overall volcanic cloud predictability. It might also be essential to designing geoengineering technologies based on the injection of aerosol precursors in the lower stratosphere. © 2021. The Authors.
英文关键词ash; explosive eruptions; SO2; sulfate; volcanic cloud
语种英语
来源期刊Journal of Geophysical Research: Atmospheres
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/185221
作者单位King Abdullah University of Science and Technology, Thuwal, Saudi Arabia; Max Planck Institute for Chemistry, Mainz, Germany; CIRES, University of Colorado, Boulder, CO, United States; NOAA Earth Systems Research Laboratory, Boulder, CO, United States; Atmospheric and Environmental Research, Lexington, MA, United States
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Stenchikov G.,Ukhov A.,Osipov S.,et al. How Does a Pinatubo-Size Volcanic Cloud Reach the Middle Stratosphere?[J],2021,126(10).
APA Stenchikov G..,Ukhov A..,Osipov S..,Ahmadov R..,Grell G..,...&Iacono M..(2021).How Does a Pinatubo-Size Volcanic Cloud Reach the Middle Stratosphere?.Journal of Geophysical Research: Atmospheres,126(10).
MLA Stenchikov G.,et al."How Does a Pinatubo-Size Volcanic Cloud Reach the Middle Stratosphere?".Journal of Geophysical Research: Atmospheres 126.10(2021).
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