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DOI10.1073/pnas.2020583118
Sea spray aerosol concentration modulated by sea surface temperature
Liu S.; Liu C.-C.; Froyd K.D.; Schill G.P.; Murphy D.M.; Bui T.P.; Dean-Day J.M.; Weinzierl B.; Dollner M.; Diskin G.S.; Chen G.; Gao R.-S.
发表日期2021
ISSN00278424
卷号118期号:9
英文摘要Natural aerosols in pristine regions form the baseline used to evaluate the impact of anthropogenic aerosols on climate. Sea spray aerosol (SSA) is a major component of natural aerosols. Despite its importance, the abundance of SSA is poorly constrained. It is generally accepted that wind-driven wave breaking is the principle governing SSA production. This mechanism alone, however, is insufficient to explain the variability of SSA concentration at given wind speed. The role of other parameters, such as sea surface temperature (SST), remains controversial. Here, we show that higher SST promotes SSA mass generation at a wide range of wind speed levels over the remote Pacific and Atlantic Oceans, in addition to demonstrating the wind-driven SSA production mechanism. The results are from a global scale dataset of airborne SSA measurements at 150 to 200 m above the ocean surface during the NASA Atmospheric Tomography Mission. Statistical analysis suggests that accounting for SST greatly enhances the predictability of the observed SSA concentration compared to using wind speed alone. Our results support implementing SST into SSA source functions in global models to better understand the atmospheric burdens of SSA. © This open access article is distributed under Creative Commons Attribution-NonCommercialNoDerivatives License 4.0 (CC BY-NC-ND).
英文关键词Marine aerosols; NASA ATom; Sea surface temperature; Wind speed
语种英语
scopus关键词aerosol; article; Atlantic Ocean; controlled study; sea surface temperature; tomography; wind speed
来源期刊Proceedings of the National Academy of Sciences of the United States of America
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/180450
作者单位Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, United States; NOAA Chemical Sciences Laboratory, Boulder, CO 80305, United States; School of Earth and Space Sciences, University of Science and Technology of China, Hefei, Anhui, 230026, China; Atmospheric Science Branch, NASA Ames Research Center, Moffett Field, CA 94035, United States; Bay Area Environmental Research Institute, Moffett Field, CA 94035, United States; University of Vienna, Faculty of Physics, Aerosol Physics and Environmental Physics, Vienna, 1090, Austria; Chemistry and Dynamics Branch, Science Directorate, NASA Langley Research Center, Hampton, VA 23681, United States; Research Division, California Air Resources Board, Sacramento, CA 95814, United States
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GB/T 7714
Liu S.,Liu C.-C.,Froyd K.D.,et al. Sea spray aerosol concentration modulated by sea surface temperature[J],2021,118(9).
APA Liu S..,Liu C.-C..,Froyd K.D..,Schill G.P..,Murphy D.M..,...&Gao R.-S..(2021).Sea spray aerosol concentration modulated by sea surface temperature.Proceedings of the National Academy of Sciences of the United States of America,118(9).
MLA Liu S.,et al."Sea spray aerosol concentration modulated by sea surface temperature".Proceedings of the National Academy of Sciences of the United States of America 118.9(2021).
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