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DOI10.1038/s41612-018-0045-5
Response of surface ozone over the continental United States to UV radiation declines from the expected recovery of stratospheric ozone
Hodzic A.; Madronich S.
发表日期2018
ISSN23973722
卷号1期号:1
英文摘要The response of surface ozone concentrations to decreases in ultraviolet (UV) radiation that are expected from the recovery of stratospheric ozone by the end of the twenty-first century is examined with the regional WRF–Chem model. The study is performed over the continental United States for the summer of 2010 at 12 km horizontal resolution which, compared to previous studies, allows a better separation of chemical regimes that exhibit opposite responses to UV radiation changes. Our results show that on the regional scale, surface ozone is expected to increase by 0.5 to 1 ppb due to its slower destruction, while the opposite can be seen in the vicinity of some urban centers where ozone concentrations could decrease by up to 1 ppb due to its slower photochemical production. Geographic overlay with population shows however a relatively small net increase in exposure of ~ 0.4 ppb, with an asymmetric distribution characterized by some disbenefit to the majority of the US population and a benefit to a relatively small fraction (~4%) of population. © 2018, The Author(s).
语种英语
scopus关键词atmospheric chemistry; atmospheric modeling; concentration (composition); ozone; photochemistry; stratosphere; ultraviolet radiation; United States
来源期刊npj Climate and Atmospheric Science
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/178198
作者单位Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, United States; Laboratoire d’Aérologie Université de Toulouse, CNRS, UPS, Toulouse, France
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Hodzic A.,Madronich S.. Response of surface ozone over the continental United States to UV radiation declines from the expected recovery of stratospheric ozone[J],2018,1(1).
APA Hodzic A.,&Madronich S..(2018).Response of surface ozone over the continental United States to UV radiation declines from the expected recovery of stratospheric ozone.npj Climate and Atmospheric Science,1(1).
MLA Hodzic A.,et al."Response of surface ozone over the continental United States to UV radiation declines from the expected recovery of stratospheric ozone".npj Climate and Atmospheric Science 1.1(2018).
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