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DOI10.3390/atmos10060330
Pollution events at the high-altitude mountain site Zugspitze-Schneefernerhaus (2670 m a.s.l.); Germany
Ghasemifard H.; Vogel F.R.; Yuan Y.; Luepke M.; Chen J.; Ries L.; Leuchner M.; Schunk C.; Vardag S.N.; Menzel A.
发表日期2019
ISSN20734433
卷号10期号:6
英文摘要Within the CO2 time series measured at the Environmental Research Station Schneefernerhaus (UFS), Germany, as part of the Global Atmospheric Watch (GAW) program, pollution episodes are traced back to local and regional emissions, identified by δ13C(CO2) as well as ratios of CO and CH4 to CO2 mixing ratios. Seven episodes of sudden enhancements in the tropospheric CO2 mixing ratio are identified in the measurements of mixing/isotopic ratios during five winter months from October 2012 to February 2013. The short-term CO2 variations are closely correlated with changes in CO and CH4 mixing ratios, achieving mean values of 6.0 ± 0.2 ppb/ppm for CO/CO2 and 6.0 ± 0.1 ppb/ppm for CH4/CO2. The estimated isotopic signature of CO2 sources (δs) ranges between -35‰ and -24‰, with higher values indicating contributions from coal combustion or wood burning, and lower values being the result of natural gas or gasoline. Moving Keeling plots with site-specific data selection criteria are applied to detect these pollution events. Furthermore, the HYSPLIT trajectory model is utilized to identify the trajectories during periods with CO2 peak events. Short trajectories are found covering Western and Central Europe, while clean air masses flow from the Atlantic Ocean and the Arctic Ocean. by the authors.
英文关键词Air pollutant transport; Atmospheric CO2 mixing ratio; Emission ratio; Environmental Research Station Schneefernerhaus (UFS); Global Atmospheric Watch (GAW); HYSPLIT model; Isotopic CO2
scopus关键词Atmospheric movements; Coal combustion; Isotopes; Mixing; Pollution; Site selection; Trajectories; Watches; Air pollutant transport; Emission ratio; Environmental researches; Global atmospheric watches; HYSPLIT model; Isotopic CO2; Mixing ratios; Carbon dioxide; atmospheric pollution; carbon dioxide; concentration (composition); emission control; mountain environment; pollutant transport; research; Germany
来源期刊Atmosphere
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/176417
作者单位Professorship of Ecoclimatology, Technische Universität München, Freising, 85354, Germany; Climate Research Division, Environment and Climate Change Canada, Toronto, ON M3H 5T4, Canada; Professorship of Environmental Sensing and Modeling, Technische Universität München, Munich, 80333, Germany; Institute for Advanced Study, Technische Universität München, Garching, 85748, Germany; German Environment Agency (UBA), Zugspitze, 82475, Germany; Physical Geography and Climatology, RWTH Aachen University, Aachen, 52056, Germany; Department for Safety and Radiation Protection, Technische Universität München, Garching, 85748, Germany; Heidelberg Center for the Environment, Universität Heidelberg, Heidelberg, 69120, Germany
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Ghasemifard H.,Vogel F.R.,Yuan Y.,et al. Pollution events at the high-altitude mountain site Zugspitze-Schneefernerhaus (2670 m a.s.l.); Germany[J],2019,10(6).
APA Ghasemifard H..,Vogel F.R..,Yuan Y..,Luepke M..,Chen J..,...&Menzel A..(2019).Pollution events at the high-altitude mountain site Zugspitze-Schneefernerhaus (2670 m a.s.l.); Germany.Atmosphere,10(6).
MLA Ghasemifard H.,et al."Pollution events at the high-altitude mountain site Zugspitze-Schneefernerhaus (2670 m a.s.l.); Germany".Atmosphere 10.6(2019).
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