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DOI10.1029/2020GL088858
Efficient Vertical Transport of Black Carbon in the Planetary Boundary Layer
Liu D.; Hu K.; Zhao D.; Ding S.; Wu Y.; Zhou C.; Yu C.; Tian P.; Liu Q.; Bi K.; Wu Y.; Hu B.; Ji D.; Kong S.; Ouyang B.; He H.; Huang M.; Ding D.
发表日期2020
ISSN 0094-8276
卷号47期号:15
英文摘要Vertical distribution of black carbon (BC) determines the layer where its heating impacts exert. This study presents continuous and simultaneous measurements at surface and on a mountain site above the wintertime planetary boundary layer influenced by uplifted surface anthropogenic emissions. BC was observed efficiently transported upwards by daytime convective mixing. However, this vertical transport was less for other particulate masses. An about twofold higher BC mass fraction was thus present at mountain than surface, hereby a lowered single-scattering albedo (SSA) by 0.06. This may be caused by the evaporative loss of condensed semivolatile materials, prevailing the secondary particulate formation, in a cleaner environment containing less precursors. The elevated BC mass corresponded with the most intensive solar radiation at midday, wielding more heating impacts over the planetary boundary layer (PBL). This phenomenon may apply to other remote regions where a reduced SSA will introduce more positive radiative effects. © 2020. American Geophysical Union. All Rights Reserved.
英文关键词Atmospheric thermodynamics; Carbon; Particulate emissions; Solar radiation; Anthropogenic emissions; Planetary boundary layers; Secondary particulates; Semi-volatile materials; Simultaneous measurement; Single scattering albedo; Vertical distributions; Vertical transports; Boundary layers; albedo; anthropogenic effect; black carbon; boundary layer; convective system; emission; mixing; scattering; vertical distribution; winter
语种英语
来源期刊Geophysical Research Letters
文献类型期刊论文
条目标识符http://gcip.llas.ac.cn/handle/2XKMVOVA/170059
作者单位Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, China; Beijing Weather Modification Office, Beijing, China; Key Laboratory of Regional Climate-Environment for Temperate East Asia (RCE-TEA), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China; Centre for Atmospheric Sciences, School of Earth and Environmental Sciences, University of Manchester, Manchester, United Kingdom; State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China; Department of Atmospheric Sciences, School of Environmental Studies, China University of Geosciences, Wuhan, China; Lancaster Environment Centre, Library Avenue, Lancaster University, Lancaster, United Kingdom
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GB/T 7714
Liu D.,Hu K.,Zhao D.,et al. Efficient Vertical Transport of Black Carbon in the Planetary Boundary Layer[J],2020,47(15).
APA Liu D..,Hu K..,Zhao D..,Ding S..,Wu Y..,...&Ding D..(2020).Efficient Vertical Transport of Black Carbon in the Planetary Boundary Layer.Geophysical Research Letters,47(15).
MLA Liu D.,et al."Efficient Vertical Transport of Black Carbon in the Planetary Boundary Layer".Geophysical Research Letters 47.15(2020).
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